by Martinelli, Leonardo, Betto, Davide, Kummer, Kurt, Arpaia, Riccardo, Braicovich, Lucio, Di Castro, Daniele, Brookes, Nicholas B., Moretti Sala, Marco and Ghiringhelli, Giacomo
Abstract:
We use resonant inelastic x-ray scattering (RIXS) to investigate the magnetic dynamics of the infinite-layer cuprate CaCuO2. We find that close to the (1/2,0) point, the single magnon decays into a broad continuum of excitations accounting for about 80% of the total magnetic spectral weight. Polarization-resolved RIXS spectra reveal the overwhelming dominance of the spin-flip (?S=1) character of this continuum with respect to the ?S=0 multimagnon contributions. Moreover, its incident-energy dependence is identical to that of the magnon, supporting a common physical origin. We propose that the continuum originates from the decay of the magnon into spinon pairs, and we relate it to the exceptionally high ring exchange Jc J1 of CaCuO2. In the infinite-layer cuprates, long-range and multisite hopping integrals are very important, and they amplify the 2D quantum magnetism effects in spite of the 3D antiferromagnetic Néel order. © 2022 authors. Published by the American Physical Society.
Reference:
Fractional Spin Excitations in the Infinite-Layer Cuprate CaCuO2 (Martinelli, Leonardo, Betto, Davide, Kummer, Kurt, Arpaia, Riccardo, Braicovich, Lucio, Di Castro, Daniele, Brookes, Nicholas B., Moretti Sala, Marco and Ghiringhelli, Giacomo), In Physical Review X, volume 12, 2022.
Bibtex Entry:
@ARTICLE{Martinelli2022,
	author = {Martinelli, Leonardo and Betto, Davide and Kummer, Kurt and Arpaia, Riccardo and Braicovich, Lucio and Di Castro, Daniele and Brookes, Nicholas B. and Moretti Sala, Marco and Ghiringhelli, Giacomo},
	title = {Fractional Spin Excitations in the Infinite-Layer Cuprate CaCuO2},
	year = {2022},
	journal = {Physical Review X},
	volume = {12},
	number = {2},
	doi = {10.1103/PhysRevX.12.021041},
	url = {https://www.scopus.com/inward/record.uri?eid=2-s2.0-85131349230&doi=10.1103%2fPhysRevX.12.021041&partnerID=40&md5=b631e4eadc5f95f148ade64b2123baf1},
	abstract = {We use resonant inelastic x-ray scattering (RIXS) to investigate the magnetic dynamics of the infinite-layer cuprate CaCuO2. We find that close to the (1/2,0) point, the single magnon decays into a broad continuum of excitations accounting for about 80% of the total magnetic spectral weight. Polarization-resolved RIXS spectra reveal the overwhelming dominance of the spin-flip (?S=1) character of this continuum with respect to the ?S=0 multimagnon contributions. Moreover, its incident-energy dependence is identical to that of the magnon, supporting a common physical origin. We propose that the continuum originates from the decay of the magnon into spinon pairs, and we relate it to the exceptionally high ring exchange Jc~J1 of CaCuO2. In the infinite-layer cuprates, long-range and multisite hopping integrals are very important, and they amplify the 2D quantum magnetism effects in spite of the 3D antiferromagnetic Néel order.  © 2022 authors. Published by the American Physical Society.},
	type = {Article},
	publication_stage = {Final},
	source = {Scopus},
	note = {All Open Access, Gold Open Access, Green Open Access}
}

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