by Suzuki, Hakuto, Minola, Matteo, Lu, Yi, Peng, Yingying and Fumagalli, Roberto, Lefrancois, Emilie, Loew, Toshinao, Porras, Juan, Kummer, Kurt, Betto, Davide, Ishida, Shigeyuki and Eisaki, Hiroshi, Hu, Cheng, Zhou, Xingjiang, Haverkort, Maurits W., Brookes, Nicholas B., Braicovich, Lucio, Ghiringhelli, Giacomo, Le Tacon, Matthieu and Keimer, Bernhard
Abstract:
The determination of the symmetry of the energy gap is crucial for research on the microscopic mechanisms of unconventional superconductivity. Here, we demonstrate experimentally that high-resolution resonant inelastic X-ray scattering at the Cu L-3 edge can serve as a momentum-resolved, bulk-sensitive probe of the superconducting gap. We studied two optimally doped cuprates Bi2Sr2CaCu2O8+delta and Bi2Sr2Ca2Cu3O10+delta, in which we observe a strongly momentum dependent reduction of the spectral weight upon entering the superconducting state, with a maximum for momenta connecting antinodal regions of the Fermi surface. Based on a comparison with the calculated charge susceptibility and electronic Raman scattering data, we interpret our observation as a renormalization of the non-local charge susceptibility due to the superconducting gap opening. Our data demonstrate the methodological potential of resonant inelastic X-ray scattering as a versatile probe of the energy gap of high-temperature superconductors, including buried interfaces in heterostructures which are inaccessible to angle-resolved photoemission spectroscopy.
Reference:
Probing the energy gap of high-temperature cuprate superconductors by resonant inelastic x-ray scattering (Suzuki, Hakuto, Minola, Matteo, Lu, Yi, Peng, Yingying and Fumagalli, Roberto, Lefrancois, Emilie, Loew, Toshinao, Porras, Juan, Kummer, Kurt, Betto, Davide, Ishida, Shigeyuki and Eisaki, Hiroshi, Hu, Cheng, Zhou, Xingjiang, Haverkort, Maurits W., Brookes, Nicholas B., Braicovich, Lucio, Ghiringhelli, Giacomo, Le Tacon, Matthieu and Keimer, Bernhard), In NPJ QUANTUM MATERIALS, NATURE PUBLISHING GROUP, volume 3, 2018.
Bibtex Entry:
@article{ ISI:000463712700001, Author = {Suzuki, Hakuto and Minola, Matteo and Lu, Yi and Peng, Yingying and Fumagalli, Roberto and Lefrancois, Emilie and Loew, Toshinao and Porras, Juan and Kummer, Kurt and Betto, Davide and Ishida, Shigeyuki and Eisaki, Hiroshi and Hu, Cheng and Zhou, Xingjiang and Haverkort, Maurits W. and Brookes, Nicholas B. and Braicovich, Lucio and Ghiringhelli, Giacomo and Le Tacon, Matthieu and Keimer, Bernhard}, Title = {{Probing the energy gap of high-temperature cuprate superconductors by resonant inelastic x-ray scattering}}, Journal = {{NPJ QUANTUM MATERIALS}}, Year = {{2018}}, Volume = {{3}}, Month = {{DEC 14}}, Abstract = {{The determination of the symmetry of the energy gap is crucial for research on the microscopic mechanisms of unconventional superconductivity. Here, we demonstrate experimentally that high-resolution resonant inelastic X-ray scattering at the Cu L-3 edge can serve as a momentum-resolved, bulk-sensitive probe of the superconducting gap. We studied two optimally doped cuprates Bi2Sr2CaCu2O8+delta and Bi2Sr2Ca2Cu3O10+delta, in which we observe a strongly momentum dependent reduction of the spectral weight upon entering the superconducting state, with a maximum for momenta connecting antinodal regions of the Fermi surface. Based on a comparison with the calculated charge susceptibility and electronic Raman scattering data, we interpret our observation as a renormalization of the non-local charge susceptibility due to the superconducting gap opening. Our data demonstrate the methodological potential of resonant inelastic X-ray scattering as a versatile probe of the energy gap of high-temperature superconductors, including buried interfaces in heterostructures which are inaccessible to angle-resolved photoemission spectroscopy.}}, Publisher = {{NATURE PUBLISHING GROUP}}, Address = {{MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Suzuki, H; Keimer, B (Corresponding Author), Max Planck Inst Festkorperforsch, Heisenbergstr 1, D-70569 Stuttgart, Germany. Suzuki, Hakuto; Minola, Matteo; Lu, Yi; Lefrancois, Emilie; Loew, Toshinao; Porras, Juan; Keimer, Bernhard, Max Planck Inst Festkorperforsch, Heisenbergstr 1, D-70569 Stuttgart, Germany. Peng, Yingying; Fumagalli, Roberto; Braicovich, Lucio; Ghiringhelli, Giacomo, Politecn Milan, Dipartimento Fis, Piazza Leonardo da Vinci 32, I-20133 Milan, Italy. Kummer, Kurt; Betto, Davide; Brookes, Nicholas B.; Braicovich, Lucio, European Synchrotron Radiat Facil, 71 Ave Martyrs, F-38043 Grenoble, France. Ishida, Shigeyuki; Eisaki, Hiroshi, Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. Hu, Cheng; Zhou, Xingjiang, Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. Haverkort, Maurits W., Heidelberg Univ, Inst Theoret Phys, Philosophenweg 19, D-69120 Heidelberg, Germany. Le Tacon, Matthieu, Karlsruher Inst Technol, Inst Festkorperphys, Hermann v Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany.}}, DOI = {{10.1038/s41535-018-0139-7}}, Article-Number = {{65}}, EISSN = {{2397-4648}}, Keywords-Plus = {{ELECTRONIC RAMAN-SCATTERING; INPLANE SPECTRAL WEIGHT; SINGLE-CRYSTAL GROWTH; T-C; DOPING DEPENDENCE; EXCITATIONS; BI2SR2CACU2O8; STATE}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Quantum Science & Technology; Physics, Applied; Physics, Condensed Matter}}, Author-Email = {{h.suzuki@fkf.mpg.de b.keimer@fkf.mpg.de}}, ResearcherID-Numbers = {{HU, Cheng/AAZ-7539-2020 Lefrancois, Emilie/Q-4316-2019 Lu, Yi/G-9881-2014 , Le Tacon Matthieu/D-8023-2011 Ghiringhelli, Giacomo/D-1159-2014 Ishida, Shigeyuki/L-6231-2018 peng, yingying/K-1805-2015 Haverkort, Maurits W./D-2319-2009 }}, ORCID-Numbers = {{HU, Cheng/0000-0003-2335-7806 Lefrancois, Emilie/0000-0002-8959-7848 Lu, Yi/0000-0001-9445-641X , Le Tacon Matthieu/0000-0002-5838-3724 Ghiringhelli, Giacomo/0000-0003-0867-7748 Ishida, Shigeyuki/0000-0001-9445-8079 Braicovich, Lucio/0000-0001-6548-9140 peng, yingying/0000-0002-2657-3590 Suzuki, Hakuto/0000-0003-2973-0579 Haverkort, Maurits W./0000-0002-7216-3146 Minola, Matteo/0000-0003-4084-0664}}, Funding-Acknowledgement = {{JSPSMinistry of Education, Culture, Sports, Science and Technology, Japan (MEXT)Japan Society for the Promotion of Science; Alexander von Humboldt FoundationAlexander von Humboldt Foundation; Fondazione CARIPLOFondazione Cariplo; Regione Lombardia, Italy, through the ERC-P-ReXS project {[}2016-0790]}}, Funding-Text = {{H.S. acknowledges financial support from the JSPS Research Fellowship for Research Abroad. M.M. was partially supported by the Alexander von Humboldt Foundation. G.G. and Y.Y.P. were partially supported by the Fondazione CARIPLO and Regione Lombardia, Italy, through the ERC-P-ReXS project (2016-0790).}}, Number-of-Cited-References = {{42}}, Times-Cited = {{5}}, Usage-Count-Last-180-days = {{2}}, Usage-Count-Since-2013 = {{7}}, Journal-ISO = {{npj Quantum Mater.}}, Doc-Delivery-Number = {{HS2SQ}}, Unique-ID = {{ISI:000463712700001}}, OA = {{DOAJ Gold, Green Published}}, DA = {{2020-12-22}}, }
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