by Hepting, M., Chaix, L., Huang, E. W., Fumagalli, R., Peng, Y. Y., Moritz, B., Kummer, K., Brookes, N. B., Lee, W. C., Hashimoto, M., Sarkar, T., He, J-F, Rotundu, C. R., Lee, Y. S., Greene, R. L., Braicovich, L., Ghiringhelli, G. and Shen, Z. X., Devereaux, T. P. and Lee, W. S.
Abstract:
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional(1,2), but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state(3,4) within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides(5-7) reveals their charge origin, that is, without mixing with magnetic components(5-7). The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought `acoustic plasmon, which is a branch of distinct charge collective modes predicted for layered systems(8-12) and argued to play a substantial part in mediating high-temperature superconductivity(10-12).
Reference:
Three-dimensional collective charge excitations in electron-doped copper oxide superconductors (Hepting, M., Chaix, L., Huang, E. W., Fumagalli, R., Peng, Y. Y., Moritz, B., Kummer, K., Brookes, N. B., Lee, W. C., Hashimoto, M., Sarkar, T., He, J-F, Rotundu, C. R., Lee, Y. S., Greene, R. L., Braicovich, L., Ghiringhelli, G. and Shen, Z. X., Devereaux, T. P. and Lee, W. S.), In NATURE, NATURE PUBLISHING GROUP, volume 563, 2018.
Bibtex Entry:
@article{ ISI:000450048400054, Author = {Hepting, M. and Chaix, L. and Huang, E. W. and Fumagalli, R. and Peng, Y. Y. and Moritz, B. and Kummer, K. and Brookes, N. B. and Lee, W. C. and Hashimoto, M. and Sarkar, T. and He, J-F and Rotundu, C. R. and Lee, Y. S. and Greene, R. L. and Braicovich, L. and Ghiringhelli, G. and Shen, Z. X. and Devereaux, T. P. and Lee, W. S.}, Title = {{Three-dimensional collective charge excitations in electron-doped copper oxide superconductors}}, Journal = {{NATURE}}, Year = {{2018}}, Volume = {{563}}, Number = {{7731}}, Pages = {{374+}}, Month = {{NOV 15}}, Abstract = {{High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional(1,2), but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state(3,4) within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides(5-7) reveals their charge origin, that is, without mixing with magnetic components(5-7). The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought `acoustic plasmon, which is a branch of distinct charge collective modes predicted for layered systems(8-12) and argued to play a substantial part in mediating high-temperature superconductivity(10-12).}}, Publisher = {{NATURE PUBLISHING GROUP}}, Address = {{MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Shen, ZX; Devereaux, TP; Lee, WS (Corresponding Author), Stanford Inst Mat & Energy Sci, SLAG Natl Accelerator Lab, Menlo Pk, CA 94025 USA. Shen, ZX; Devereaux, TP; Lee, WS (Corresponding Author), Stanford Univ, Menlo Pk, CA 94025 USA. Hepting, M.; Chaix, L.; Huang, E. W.; Moritz, B.; He, J-F; Rotundu, C. R.; Lee, Y. S.; Shen, Z. X.; Devereaux, T. P.; Lee, W. S., Stanford Inst Mat & Energy Sci, SLAG Natl Accelerator Lab, Menlo Pk, CA 94025 USA. Hepting, M.; Chaix, L.; Huang, E. W.; Moritz, B.; He, J-F; Rotundu, C. R.; Lee, Y. S.; Shen, Z. X.; Devereaux, T. P.; Lee, W. S., Stanford Univ, Menlo Pk, CA 94025 USA. Huang, E. W., Stanford Univ, Dept Phys, Stanford, CA 94305 USA. Fumagalli, R.; Peng, Y. Y.; Braicovich, L.; Ghiringhelli, G., Politecn Milan, Dipartimento Fis, Milan, Italy. Kummer, K.; Brookes, N. B.; Braicovich, L., ESRF, Grenoble, France. Lee, W. C., SUNY Binghamton, Dept Phys, Binghamton, NY 13902 USA. Hashimoto, M., SLAG Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA USA. Sarkar, T.; Greene, R. L., Univ Maryland, Ctr Nanophys & Adv Mat, Dept Phys, College Pk, MD 20742 USA. Ghiringhelli, G., Politecn Milan, CNR SPIN, Milan, Italy. Chaix, L., Univ Grenoble Alpes, CNRS, Inst Neel, Grenoble, France. Peng, Y. Y., Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. Peng, Y. Y., Univ Illinois, Seitz Mat Res Lab, Urbana, IL 61801 USA. He, J-F, Univ Sci & Technol China, Dept Phys, Hefei, Anhui, Peoples R China.}}, DOI = {{10.1038/s41586-018-0648-3}}, ISSN = {{0028-0836}}, EISSN = {{1476-4687}}, Keywords-Plus = {{CUPRATE SUPERCONDUCTIVITY; ENERGY; PLASMONS; GAS; ELECTRODYNAMICS}}, Research-Areas = {{Science & Technology - Other Topics}}, Web-of-Science-Categories = {{Multidisciplinary Sciences}}, Author-Email = {{zxshen@stanford.edu tpd@stanford.edu leews@stanford.edu}}, ResearcherID-Numbers = {{Sarkar, Tarapada/J-7879-2019 Hepting, Matthias/AAH-1592-2019 Ghiringhelli, Giacomo/D-1159-2014 Moritz, Brian J/D-7505-2015 Brookes, Nicholas B/C-6718-2019 }}, ORCID-Numbers = {{Sarkar, Tarapada/0000-0002-4204-4250 Hepting, Matthias/0000-0002-5824-8901 Ghiringhelli, Giacomo/0000-0003-0867-7748 Moritz, Brian J/0000-0002-3747-8484 Brookes, Nicholas B/0000-0002-1342-9530 Braicovich, Lucio/0000-0001-6548-9140 Huang, Edwin/0000-0002-6250-9529 Chaix, Laura/0000-0002-6757-9040 He, Junfeng/0000-0001-5584-9827}}, Funding-Acknowledgement = {{US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering DivisionUnited States Department of Energy (DOE) {[}DE-AC02-76SF00515]; Department of Energy, SLAC Laboratory Directed Research and Development {[}DE-AC02-76SF00515]; ERC-P-ReXS project of the Fondazione CARIPLOFondazione Cariplo {[}2016-0790]; Regione Lombardia, in Italy; NSFNational Science Foundation (NSF) {[}DMR-1708334]; US DOEUnited States Department of Energy (DOE) {[}DE-AC02-05CH11231]}}, Funding-Text = {{This work is supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, under contract DE-AC02-76SF00515. L.C. acknowledges support from the Department of Energy, SLAC Laboratory Directed Research and Development funder contract under DE-AC02-76SF00515. RIXS data were taken at beamline ID32 of the European Synchrotron Radiation Facility (ESRF, Grenoble, France) using the ERIXS spectrometer designed jointly by the ESRF and the Politecnico di Milano. G.G. and Y.Y.P. were supported by the by ERC-P-ReXS project (2016-0790) of the Fondazione CARIPLO and Regione Lombardia, in Italy. R.L.G. and T.S. acknowledge support from NSF award DMR-1708334. Computational work was performed on the Sherlock cluster at Stanford University and on resources of the National Energy Research Scientific Computing Center, supported by the US DOE under contract number DE-AC02-05CH11231.}}, Number-of-Cited-References = {{40}}, Times-Cited = {{31}}, Usage-Count-Last-180-days = {{14}}, Usage-Count-Since-2013 = {{105}}, Journal-ISO = {{Nature}}, Doc-Delivery-Number = {{HA2EY}}, Unique-ID = {{ISI:000450048400054}}, DA = {{2020-12-22}}, }
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