by Hepting, M., Chaix, L., Huang, E. W., Fumagalli, R., Peng, Y. Y., Moritz, B., Kummer, K., Brookes, N. B., Lee, W. C., Hashimoto, M., Sarkar, T., He, J-F, Rotundu, C. R., Lee, Y. S., Greene, R. L., Braicovich, L., Ghiringhelli, G. and Shen, Z. X., Devereaux, T. P. and Lee, W. S.
Abstract:
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional(1,2), but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state(3,4) within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides(5-7) reveals their charge origin, that is, without mixing with magnetic components(5-7). The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought `acoustic plasmon, which is a branch of distinct charge collective modes predicted for layered systems(8-12) and argued to play a substantial part in mediating high-temperature superconductivity(10-12).
Reference:
Three-dimensional collective charge excitations in electron-doped copper oxide superconductors (Hepting, M., Chaix, L., Huang, E. W., Fumagalli, R., Peng, Y. Y., Moritz, B., Kummer, K., Brookes, N. B., Lee, W. C., Hashimoto, M., Sarkar, T., He, J-F, Rotundu, C. R., Lee, Y. S., Greene, R. L., Braicovich, L., Ghiringhelli, G. and Shen, Z. X., Devereaux, T. P. and Lee, W. S.), In NATURE, NATURE PUBLISHING GROUP, volume 563, 2018.
Bibtex Entry:
@article{ ISI:000450048400054,
Author = {Hepting, M. and Chaix, L. and Huang, E. W. and Fumagalli, R. and Peng,
Y. Y. and Moritz, B. and Kummer, K. and Brookes, N. B. and Lee, W. C.
and Hashimoto, M. and Sarkar, T. and He, J-F and Rotundu, C. R. and Lee,
Y. S. and Greene, R. L. and Braicovich, L. and Ghiringhelli, G. and
Shen, Z. X. and Devereaux, T. P. and Lee, W. S.},
Title = {{Three-dimensional collective charge excitations in electron-doped copper
oxide superconductors}},
Journal = {{NATURE}},
Year = {{2018}},
Volume = {{563}},
Number = {{7731}},
Pages = {{374+}},
Month = {{NOV 15}},
Abstract = {{High-temperature copper oxide superconductors consist of stacked CuO2
planes, with electronic band structures and magnetic excitations that
are primarily two-dimensional(1,2), but with superconducting coherence
that is three-dimensional. This dichotomy highlights the importance of
out-of-plane charge dynamics, which has been found to be incoherent in
the normal state(3,4) within the limited range of momenta accessible by
optics. Here we use resonant inelastic X-ray scattering to explore the
charge dynamics across all three dimensions of the Brillouin zone.
Polarization analysis of recently discovered collective excitations
(modes) in electron-doped copper oxides(5-7) reveals their charge
origin, that is, without mixing with magnetic components(5-7). The
excitations disperse along both the in-plane and out-of-plane
directions, revealing its three-dimensional nature. The periodicity of
the out-of-plane dispersion corresponds to the distance between
neighbouring CuO2 planes rather than to the crystallographic c-axis
lattice constant, suggesting that the interplane Coulomb interaction is
responsible for the coherent out-of-plane charge dynamics. The observed
properties are hallmarks of the long-sought `acoustic plasmon, which is
a branch of distinct charge collective modes predicted for layered
systems(8-12) and argued to play a substantial part in mediating
high-temperature superconductivity(10-12).}},
Publisher = {{NATURE PUBLISHING GROUP}},
Address = {{MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND}},
Type = {{Article}},
Language = {{English}},
Affiliation = {{Shen, ZX; Devereaux, TP; Lee, WS (Corresponding Author), Stanford Inst Mat & Energy Sci, SLAG Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
Shen, ZX; Devereaux, TP; Lee, WS (Corresponding Author), Stanford Univ, Menlo Pk, CA 94025 USA.
Hepting, M.; Chaix, L.; Huang, E. W.; Moritz, B.; He, J-F; Rotundu, C. R.; Lee, Y. S.; Shen, Z. X.; Devereaux, T. P.; Lee, W. S., Stanford Inst Mat & Energy Sci, SLAG Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
Hepting, M.; Chaix, L.; Huang, E. W.; Moritz, B.; He, J-F; Rotundu, C. R.; Lee, Y. S.; Shen, Z. X.; Devereaux, T. P.; Lee, W. S., Stanford Univ, Menlo Pk, CA 94025 USA.
Huang, E. W., Stanford Univ, Dept Phys, Stanford, CA 94305 USA.
Fumagalli, R.; Peng, Y. Y.; Braicovich, L.; Ghiringhelli, G., Politecn Milan, Dipartimento Fis, Milan, Italy.
Kummer, K.; Brookes, N. B.; Braicovich, L., ESRF, Grenoble, France.
Lee, W. C., SUNY Binghamton, Dept Phys, Binghamton, NY 13902 USA.
Hashimoto, M., SLAG Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA USA.
Sarkar, T.; Greene, R. L., Univ Maryland, Ctr Nanophys & Adv Mat, Dept Phys, College Pk, MD 20742 USA.
Ghiringhelli, G., Politecn Milan, CNR SPIN, Milan, Italy.
Chaix, L., Univ Grenoble Alpes, CNRS, Inst Neel, Grenoble, France.
Peng, Y. Y., Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA.
Peng, Y. Y., Univ Illinois, Seitz Mat Res Lab, Urbana, IL 61801 USA.
He, J-F, Univ Sci & Technol China, Dept Phys, Hefei, Anhui, Peoples R China.}},
DOI = {{10.1038/s41586-018-0648-3}},
ISSN = {{0028-0836}},
EISSN = {{1476-4687}},
Keywords-Plus = {{CUPRATE SUPERCONDUCTIVITY; ENERGY; PLASMONS; GAS; ELECTRODYNAMICS}},
Research-Areas = {{Science & Technology - Other Topics}},
Web-of-Science-Categories = {{Multidisciplinary Sciences}},
Author-Email = {{zxshen@stanford.edu
tpd@stanford.edu
leews@stanford.edu}},
ResearcherID-Numbers = {{Sarkar, Tarapada/J-7879-2019
Hepting, Matthias/AAH-1592-2019
Ghiringhelli, Giacomo/D-1159-2014
Moritz, Brian J/D-7505-2015
Brookes, Nicholas B/C-6718-2019
}},
ORCID-Numbers = {{Sarkar, Tarapada/0000-0002-4204-4250
Hepting, Matthias/0000-0002-5824-8901
Ghiringhelli, Giacomo/0000-0003-0867-7748
Moritz, Brian J/0000-0002-3747-8484
Brookes, Nicholas B/0000-0002-1342-9530
Braicovich, Lucio/0000-0001-6548-9140
Huang, Edwin/0000-0002-6250-9529
Chaix, Laura/0000-0002-6757-9040
He, Junfeng/0000-0001-5584-9827}},
Funding-Acknowledgement = {{US Department of Energy (DOE), Office of Science, Basic Energy Sciences,
Materials Sciences and Engineering DivisionUnited States Department of
Energy (DOE) {[}DE-AC02-76SF00515]; Department of Energy, SLAC
Laboratory Directed Research and Development {[}DE-AC02-76SF00515];
ERC-P-ReXS project of the Fondazione CARIPLOFondazione Cariplo
{[}2016-0790]; Regione Lombardia, in Italy; NSFNational Science
Foundation (NSF) {[}DMR-1708334]; US DOEUnited States Department of
Energy (DOE) {[}DE-AC02-05CH11231]}},
Funding-Text = {{This work is supported by the US Department of Energy (DOE), Office of
Science, Basic Energy Sciences, Materials Sciences and Engineering
Division, under contract DE-AC02-76SF00515. L.C. acknowledges support
from the Department of Energy, SLAC Laboratory Directed Research and
Development funder contract under DE-AC02-76SF00515. RIXS data were
taken at beamline ID32 of the European Synchrotron Radiation Facility
(ESRF, Grenoble, France) using the ERIXS spectrometer designed jointly
by the ESRF and the Politecnico di Milano. G.G. and Y.Y.P. were
supported by the by ERC-P-ReXS project (2016-0790) of the Fondazione
CARIPLO and Regione Lombardia, in Italy. R.L.G. and T.S. acknowledge
support from NSF award DMR-1708334. Computational work was performed on
the Sherlock cluster at Stanford University and on resources of the
National Energy Research Scientific Computing Center, supported by the
US DOE under contract number DE-AC02-05CH11231.}},
Number-of-Cited-References = {{40}},
Times-Cited = {{31}},
Usage-Count-Last-180-days = {{14}},
Usage-Count-Since-2013 = {{105}},
Journal-ISO = {{Nature}},
Doc-Delivery-Number = {{HA2EY}},
Unique-ID = {{ISI:000450048400054}},
DA = {{2020-12-22}},
}
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