by Calder, S., Vale, J. G., Bogdanov, N., Donnerer, C. and Pincini, D., Sala, M. Moretti, Liu, X., Upton, M. H., Casa, D., Shi, Y. G., Tsujimoto, Y., Yamaura, K., Hill, J. P. and van den Brink, J., McMorrow, D. F. and Christianson, A. D.
Abstract:
NaOsO3 hosts a rare manifestation of a metal-insulator transition driven by magnetic correlations, placing the magnetic exchange interactions in a central role. We use resonant inelastic x-ray scattering to directly probe these magnetic exchange interactions. A dispersive and strongly gapped (58 meV) excitation is observed, indicating appreciable spin-orbit coupling in this 5d(3) system. The excitation is well described within a minimal model Hamiltonian with strong anisotropy and Heisenberg exchange (J(1) = J(2) = 13.9 meV). The observed behavior places NaOsO3 on the boundary between localized and itinerant magnetism.
Reference:
Strongly gapped spin-wave excitation in the insulating phase of NaOsO3 (Calder, S., Vale, J. G., Bogdanov, N., Donnerer, C. and Pincini, D., Sala, M. Moretti, Liu, X., Upton, M. H., Casa, D., Shi, Y. G., Tsujimoto, Y., Yamaura, K., Hill, J. P. and van den Brink, J., McMorrow, D. F. and Christianson, A. D.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 95, 2017.
Bibtex Entry:
@article{ ISI:000398728100004, Author = {Calder, S. and Vale, J. G. and Bogdanov, N. and Donnerer, C. and Pincini, D. and Sala, M. Moretti and Liu, X. and Upton, M. H. and Casa, D. and Shi, Y. G. and Tsujimoto, Y. and Yamaura, K. and Hill, J. P. and van den Brink, J. and McMorrow, D. F. and Christianson, A. D.}, Title = {{Strongly gapped spin-wave excitation in the insulating phase of NaOsO3}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2017}}, Volume = {{95}}, Number = {{2}}, Month = {{JAN 23}}, Abstract = {{NaOsO3 hosts a rare manifestation of a metal-insulator transition driven by magnetic correlations, placing the magnetic exchange interactions in a central role. We use resonant inelastic x-ray scattering to directly probe these magnetic exchange interactions. A dispersive and strongly gapped (58 meV) excitation is observed, indicating appreciable spin-orbit coupling in this 5d(3) system. The excitation is well described within a minimal model Hamiltonian with strong anisotropy and Heisenberg exchange (J(1) = J(2) = 13.9 meV). The observed behavior places NaOsO3 on the boundary between localized and itinerant magnetism.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Calder, S (Corresponding Author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. Calder, S.; Christianson, A. D., Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. Vale, J. G.; Donnerer, C.; Pincini, D.; McMorrow, D. F., UCL, London Ctr Nanotechnol, Gower St, London WC1E 6BT, England. Vale, J. G.; Donnerer, C.; Pincini, D.; McMorrow, D. F., UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. Vale, J. G., Ecole Polytech Fed Lausanne, Lab Quantum Magnetism, CH-1015 Lausanne, Switzerland. Bogdanov, N.; van den Brink, J., IFW Dresden, Inst Theoret Solid State Phys, D-01171 Dresden, Germany. Pincini, D., Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England. Sala, M. Moretti, European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. Liu, X.; Hill, J. P., Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. Liu, X.; Hill, J. P., Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. Liu, X.; Shi, Y. G., Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. Liu, X.; Shi, Y. G., Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. Upton, M. H.; Casa, D., Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. Shi, Y. G.; Tsujimoto, Y.; Yamaura, K., Natl Inst Mat Sci, Res Ctr Funct Mat, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan. Yamaura, K., Hokkaido Univ, Grad Sch Chem Sci & Engn, Kita Ku, North 10 West 8, Sapporo, Hokkaido 0600810, Japan. Christianson, A. D., Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.}}, DOI = {{10.1103/PhysRevB.95.020413}}, Article-Number = {{020413}}, ISSN = {{2469-9950}}, EISSN = {{2469-9969}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, Author-Email = {{caldersa@ornl.gov j.vale@ucl.ac.uk}}, ResearcherID-Numbers = {{Tsujimoto, Yoshihiro/H-6034-2012 McMorrow, Desmond Francis/M-9036-2019 Bogdanov, Nikolay A./AAD-4394-2019 Sala, Marco Moretti/H-1034-2014 van den Brink, Jeroen/E-5670-2011 McMorrow, Desmond/C-2655-2008 Moretti, Marco/AAF-9255-2019 Shi, Youguo/B-6316-2018 van den Brink, Jeroen/Y-3931-2019 }}, ORCID-Numbers = {{Tsujimoto, Yoshihiro/0000-0003-2140-3362 McMorrow, Desmond Francis/0000-0002-4947-7788 Bogdanov, Nikolay A./0000-0002-5437-4919 Sala, Marco Moretti/0000-0002-9744-9976 van den Brink, Jeroen/0000-0001-6594-9610 McMorrow, Desmond/0000-0002-4947-7788 Moretti, Marco/0000-0002-9744-9976 Pincini, Davide/0000-0002-0884-4748 YAMAURA, Kazunari/0000-0003-0390-8244 Calder, Stuart/0000-0001-8402-3741 Upton, Mary/0000-0002-9929-0487}}, Funding-Acknowledgement = {{DOE Office of Science by Argonne National LaboratoryUnited States Department of Energy (DOE) {[}DE-AC02-06CH11357]; UK Engineering and Physical Sciences Research Council (EPSRC)Engineering & Physical Sciences Research Council (EPSRC); UCL via a UCL Impact Studentship; EPFL via a UCL Impact Studentship; MOSTMinistry of Science and Technology (MOST) Korea {[}2015CB921302]; CAS of China {[}XDB07020200]; US DOE, Division of Materials Science {[}DE-SC00112704]; JSPS KAKENHIMinistry of Education, Culture, Sports, Science and Technology, Japan (MEXT)Japan Society for the Promotion of ScienceGrants-in-Aid for Scientific Research (KAKENHI) {[}15K14133, 16H04501]; Grants-in-Aid for Scientific ResearchMinistry of Education, Culture, Sports, Science and Technology, Japan (MEXT)Japan Society for the Promotion of ScienceGrants-in-Aid for Scientific Research (KAKENHI) {[}15K14133, 16H04501] Funding Source: KAKEN; Engineering and Physical Sciences Research CouncilEngineering & Physical Sciences Research Council (EPSRC) {[}EP/N034694/1, 1745233, EP/N027671/1] Funding Source: researchfish}}, Funding-Text = {{A.D.C. thanks A. E. Taylor for useful discussions. We thank C. Henriquet and R. Verbeni at the ESRF for the design and manufacture of the high-temperature stage. Preliminary measurements were performed at 9-ID-B and 30-ID (MERIX), APS, which is a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. This research used resources at the High Flux Isotope Reactor and Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory. This work in London was supported by the UK Engineering and Physical Sciences Research Council (EPSRC). J.G.V. would like to thank UCL and EPFL for financial support via a UCL Impact Studentship. X.L. acknowledges financial support from MOST (No. 2015CB921302) and CAS (No. XDB07020200) of China. Work done at Brookhaven National Laboratory was supported by US DOE, Division of Materials Science, under Contract No. DE-SC00112704. K.Y. thanks financial support from JSPS KAKENHI (15K14133 and 16H04501).}}, Number-of-Cited-References = {{23}}, Times-Cited = {{18}}, Usage-Count-Last-180-days = {{1}}, Usage-Count-Since-2013 = {{20}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{ER3VP}}, Unique-ID = {{ISI:000398728100004}}, OA = {{Green Published, Bronze}}, DA = {{2020-12-22}}, }
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