by Stornaiuolo, D., Cantoni, C., De Luca, G. M., Di Capua, R. and Di Gennaro, E., Ghiringhelli, G., Jouault, B., Marre, D. and Massarotti, D., Granozio, F. Miletto, Pallecchi, I. and Piamonteze, C., Rusponi, S., Tafuri, F. and Salluzzo, M.
Abstract:
Advances in growth technology of oxide materials allow single atomic layer control of heterostructures. In particular delta doping, a key materials’ engineering tool in today’s semiconductor technology, is now also available for oxides. Here we show that a fully electric-field-tunable spin-polarized and superconducting quasi-2D electron system (q2DES) can be artificially created by inserting a few unit cells of delta doping EuTiO3 at the interface between LaAlO3 and SrTiO3 oxides(1,2). Spin polarization emerges below the ferromagnetic transition temperature of the EuTiO3 layer (T-FM = 6-8 K) and is due to the exchange interaction between the magnetic moments of Eu-4f and of Ti-3d electrons. Moreover, in a large region of the phase diagram, superconductivity sets in from a ferromagnetic normal state. The occurrence of magnetic interactions, superconductivity and spin-orbit coupling in the same q2DES makes the LaAlO3/EuTiO3/SrTiO3 system an intriguing platform for the emergence of novel quantum phases in low-dimensional materials.
Reference:
Tunable spin polarization and superconductivity in engineered oxide interfaces (Stornaiuolo, D., Cantoni, C., De Luca, G. M., Di Capua, R. and Di Gennaro, E., Ghiringhelli, G., Jouault, B., Marre, D. and Massarotti, D., Granozio, F. Miletto, Pallecchi, I. and Piamonteze, C., Rusponi, S., Tafuri, F. and Salluzzo, M.), In NATURE MATERIALS, NATURE PUBLISHING GROUP, volume 15, 2016.
Bibtex Entry:
@article{ ISI:000370967400011,
Author = {Stornaiuolo, D. and Cantoni, C. and De Luca, G. M. and Di Capua, R. and
   Di Gennaro, E. and Ghiringhelli, G. and Jouault, B. and Marre, D. and
   Massarotti, D. and Granozio, F. Miletto and Pallecchi, I. and
   Piamonteze, C. and Rusponi, S. and Tafuri, F. and Salluzzo, M.},
Title = {{Tunable spin polarization and superconductivity in engineered oxide
   interfaces}},
Journal = {{NATURE MATERIALS}},
Year = {{2016}},
Volume = {{15}},
Number = {{3}},
Pages = {{278+}},
Month = {{MAR}},
Abstract = {{Advances in growth technology of oxide materials allow single atomic
   layer control of heterostructures. In particular delta doping, a key
   materials' engineering tool in today's semiconductor technology, is now
   also available for oxides. Here we show that a fully
   electric-field-tunable spin-polarized and superconducting quasi-2D
   electron system (q2DES) can be artificially created by inserting a few
   unit cells of delta doping EuTiO3 at the interface between LaAlO3 and
   SrTiO3 oxides(1,2). Spin polarization emerges below the ferromagnetic
   transition temperature of the EuTiO3 layer (T-FM = 6-8 K) and is due to
   the exchange interaction between the magnetic moments of Eu-4f and of
   Ti-3d electrons. Moreover, in a large region of the phase diagram,
   superconductivity sets in from a ferromagnetic normal state. The
   occurrence of magnetic interactions, superconductivity and spin-orbit
   coupling in the same q2DES makes the LaAlO3/EuTiO3/SrTiO3 system an
   intriguing platform for the emergence of novel quantum phases in
   low-dimensional materials.}},
Publisher = {{NATURE PUBLISHING GROUP}},
Address = {{MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND}},
Type = {{Article}},
Language = {{English}},
Affiliation = {{Stornaiuolo, D (Corresponding Author), Univ Naples Federico II, Dipartimento Fis, Complesso Monte Sant Angelo Via Cinthia, I-80126 Naples, Italy.
   Stornaiuolo, D; Salluzzo, M (Corresponding Author), CNR SPIN, Complesso Monte Sant Angelo Via Cinthia, I-80126 Naples, Italy.
   Stornaiuolo, D.; De Luca, G. M.; Di Capua, R.; Di Gennaro, E.; Massarotti, D., Univ Naples Federico II, Dipartimento Fis, Complesso Monte Sant Angelo Via Cinthia, I-80126 Naples, Italy.
   Stornaiuolo, D.; De Luca, G. M.; Di Capua, R.; Di Gennaro, E.; Massarotti, D.; Granozio, F. Miletto; Tafuri, F.; Salluzzo, M., CNR SPIN, Complesso Monte Sant Angelo Via Cinthia, I-80126 Naples, Italy.
   Cantoni, C., Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.
   Ghiringhelli, G., Politecn Milan, CNR SPIN, Piazza Leonardo Vinci 32, I-20133 Milan, Italy.
   Ghiringhelli, G., Politecn Milan, Dipartimento Fis, Piazza Leonardo Vinci 32, I-20133 Milan, Italy.
   Jouault, B., Univ Montpellier 2, CNRS, UMR 5221, Lab Charles Coulomb, F-34095 Montpellier, France.
   Marre, D.; Pallecchi, I., Univ Genoa, CNR SPIN, Via Dodecaneso 33, I-14146 Genoa, Italy.
   Marre, D.; Pallecchi, I., Univ Genoa, Dipartimento Fis, Via Dodecaneso 33, I-14146 Genoa, Italy.
   Piamonteze, C., Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
   Rusponi, S., Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland.
   Tafuri, F., SUN, Dipartimento Ingn Informaz, I-81031 Aversa, CE, Italy.}},
DOI = {{10.1038/NMAT4491}},
ISSN = {{1476-1122}},
EISSN = {{1476-4660}},
Keywords-Plus = {{LAALO3/SRTIO3; COEXISTENCE; MAGNETISM; ELECTRONS}},
Research-Areas = {{Chemistry; Materials Science; Physics}},
Web-of-Science-Categories  = {{Chemistry, Physical; Materials Science, Multidisciplinary; Physics,
   Applied; Physics, Condensed Matter}},
Author-Email = {{daniela.stornaiuolo@fisica.unina.it
   marco.salluzzo@spin.cnr.it}},
ResearcherID-Numbers = {{Marre, Daniele/G-5965-2014
   stornaiuolo, daniela/D-2516-2014
   Tafuri, Francesco/D-8246-2018
   Pallecchi, Ilaria/AAY-2184-2020
   GRANOZIO, FABIO MILETTO/R-9662-2017
   Di Gennaro, Emiliano/G-6311-2010
   salluzzo, marco/C-5919-2009
   Piamonteze, Cinthia/E-9740-2016
   Di Capua, Roberto/G-9622-2012
   Ghiringhelli, Giacomo/D-1159-2014
   }},
ORCID-Numbers = {{Marre, Daniele/0000-0002-6230-761X
   Tafuri, Francesco/0000-0003-0784-1454
   Pallecchi, Ilaria/0000-0001-6819-6124
   GRANOZIO, FABIO MILETTO/0000-0002-9417-7848
   Di Gennaro, Emiliano/0000-0003-4231-9776
   salluzzo, marco/0000-0001-8372-6963
   Di Capua, Roberto/0000-0003-3605-0993
   Ghiringhelli, Giacomo/0000-0003-0867-7748
   Massarotti, Davide/0000-0001-7495-362X
   jouault, benoit/0000-0002-2993-6916
   Massarotti, Davide/0000-0001-5740-0054
   Rusponi, Stefano/0000-0002-8494-5532}},
Funding-Acknowledgement = {{Ministero dell'Istruzione, dell'Universita e della RicercaMinistry of
   Education, Universities and Research (MIUR) {[}RBFR1236VV, RBAP115AYN,
   PRIN 2010-11-OXIDE]; US Department of Energy, Basic Energy Sciences,
   Materials Sciences and Engineering DivisionUnited States Department of
   Energy (DOE); CNRSCentre National de la Recherche Scientifique (CNRS)
   {[}PICS-0754]}},
Funding-Text = {{We received funding from the Ministero dell'Istruzione, dell'Universita
   e della Ricerca for the FIRB 2012 project HybridNanoDev (Grant No.
   RBFR1236VV), FIRB 2011 project `Oxides at the nanoscale:
   multifunctionality and applications' (Grant No. RBAP115AYN) and for the
   PRIN 2010-11 project (Grant No. PRIN 2010-11-OXIDE). The X-ray
   absorption measurements were performed on the EPFL/PSI X-Treme beamline
   at the Swiss Light Source, Paul Scherrer Institut, Villigen,
   Switzerland. The research of C.C. was supported by the US Department of
   Energy, Basic Energy Sciences, Materials Sciences and Engineering
   Division. The research of B.J. was supported by CNRS under PICS-0754.}},
Number-of-Cited-References = {{30}},
Times-Cited = {{55}},
Usage-Count-Last-180-days = {{7}},
Usage-Count-Since-2013 = {{220}},
Journal-ISO = {{Nat. Mater.}},
Doc-Delivery-Number = {{DE9OM}},
Unique-ID = {{ISI:000370967400011}},
DA = {{2020-12-22}},
}

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