by Salluzzo, M., Gariglio, S., Torrelles, X., Ristic, Z., Di Capua, R., Drnec, J., Sala, M. Moretti, Ghiringhelli, G. and Felici, R. and Brookes, N. B.
Abstract:
A full understanding of the mechanism of the formation of a two-dimensional electron gas (2DEG) at the interface between insulating LaAlO3 (LAO) thin films and bulk SrTiO3 (STO) crystals is a prerequisite for the full exploitation of this class of materials. Here, by using a combination of advanced X-ray synchrotron-based spectroscopic and structural measurements, it is shown that a structural and electronic reconstruction of the interface occurs before the realization of the 2DEG.
Reference:
Structural and Electronic Reconstructions at the LaAlO3/SrTiO3 Interface (Salluzzo, M., Gariglio, S., Torrelles, X., Ristic, Z., Di Capua, R., Drnec, J., Sala, M. Moretti, Ghiringhelli, G. and Felici, R. and Brookes, N. B.), In ADVANCED MATERIALS, WILEY-V C H VERLAG GMBH, volume 25, 2013.
Bibtex Entry:
@article{ ISI:000318040600014, Author = {Salluzzo, M. and Gariglio, S. and Torrelles, X. and Ristic, Z. and Di Capua, R. and Drnec, J. and Sala, M. Moretti and Ghiringhelli, G. and Felici, R. and Brookes, N. B.}, Title = {{Structural and Electronic Reconstructions at the LaAlO3/SrTiO3 Interface}}, Journal = {{ADVANCED MATERIALS}}, Year = {{2013}}, Volume = {{25}}, Number = {{16}}, Pages = {{2333-2338}}, Month = {{APR 24}}, Abstract = {{A full understanding of the mechanism of the formation of a two-dimensional electron gas (2DEG) at the interface between insulating LaAlO3 (LAO) thin films and bulk SrTiO3 (STO) crystals is a prerequisite for the full exploitation of this class of materials. Here, by using a combination of advanced X-ray synchrotron-based spectroscopic and structural measurements, it is shown that a structural and electronic reconstruction of the interface occurs before the realization of the 2DEG.}}, Publisher = {{WILEY-V C H VERLAG GMBH}}, Address = {{POSTFACH 101161, 69451 WEINHEIM, GERMANY}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Salluzzo, M (Corresponding Author), CNR SPIN, Complesso MonteSantangelo,Via Cinthia, I-80126 Naples, Italy. Salluzzo, M.; Ristic, Z.; Di Capua, R., CNR SPIN, I-80126 Naples, Italy. Salluzzo, M.; Ristic, Z.; Di Capua, R., Dept Phys, I-80126 Naples, Italy. Gariglio, S.; Ristic, Z., Univ Geneva, Dept Phys Mat Condensee, CH-1211 Geneva 4, Switzerland. Torrelles, X., Inst Ciencia Mat Barcelona CSIC, Barcelona 081893, Spain. Ristic, Z., Univ Belgrade, Inst Nucl Sci Vinc, Lab Atom Phys, Belgrade 11001, Serbia. Ghiringhelli, G., CNR SPIN, Milan, Italy. Ghiringhelli, G., Politecn Milan, Dept Phys, I-20133 Milan, Italy. Drnec, J.; Sala, M. Moretti; Felici, R.; Brookes, N. B., European Synchrotron Radiat Facil, F-38043 Grenoble, France.}}, DOI = {{10.1002/adma.201204555}}, ISSN = {{0935-9648}}, EISSN = {{1521-4095}}, Keywords = {{polar oxide interfaces; LAO; STO; two-dimensional electron gas (2DEG); X-ray absorption spectroscopy; surface diffraction}}, Keywords-Plus = {{GAS}}, Research-Areas = {{Chemistry; Science & Technology - Other Topics; Materials Science; Physics}}, Web-of-Science-Categories = {{Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, Author-Email = {{marco.salluzzo@spin.cnr.it}}, ResearcherID-Numbers = {{salluzzo, marco/C-5919-2009 Ristic, Zoran/AAQ-6890-2020 Drnec, Jakub/R-6369-2017 Sala, Marco Moretti/H-1034-2014 Moretti, Marco/AAF-9255-2019 Brookes, Nicholas B/C-6718-2019 felici, roberto/ABB-4459-2020 Di Capua, Roberto/G-9622-2012 Ghiringhelli, Giacomo/D-1159-2014 }}, ORCID-Numbers = {{salluzzo, marco/0000-0001-8372-6963 Ristic, Zoran/0000-0002-1854-284X Drnec, Jakub/0000-0002-9520-1555 Sala, Marco Moretti/0000-0002-9744-9976 Moretti, Marco/0000-0002-9744-9976 Brookes, Nicholas B/0000-0002-1342-9530 Di Capua, Roberto/0000-0003-3605-0993 Ghiringhelli, Giacomo/0000-0003-0867-7748 Torrelles, Xavier/0000-0002-6891-7793 felici, roberto/0000-0001-9897-5866}}, Funding-Acknowledgement = {{Spanish MICINN Agency {[}CSD2007-00041, MAT2009-09308]; European UnionEuropean Union (EU) {[}264098-MAMA]}}, Funding-Text = {{The authors acknowledge C. Richter, C. Cancellieri and D. Stornaiuolo, for growing the excellent LAO/STO films studied. We acknowledge the European Synchrothron Radiation Facility and the technical staff of the ID03, ID08 and BM25 beamlines for assistance during the experiments. Discussions with J.-M. Triscone, J. Mannhart, M. Stengel, M. Radovic, N. Plumb and A. Filippetti were very valuable for the interpretation of the experimental results. X. T. thanks the Spanish MICINN Agency for partially funding this project through Grants no. CSD2007-00041 and No. MAT2009-09308. The research leading to these results has received funding from the European Union Seventh Framework Program (FP7/2007-2013) under Grant Agreement No. 264098-MAMA.}}, Number-of-Cited-References = {{31}}, Times-Cited = {{62}}, Usage-Count-Last-180-days = {{1}}, Usage-Count-Since-2013 = {{171}}, Journal-ISO = {{Adv. Mater.}}, Doc-Delivery-Number = {{132AR}}, Unique-ID = {{ISI:000318040600014}}, DA = {{2020-12-22}}, }
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