by Achkar, A. J., Sutarto, R., Mao, X., He, F., Frano, A. and Blanco-Canosa, S., Le Tacon, M., Ghiringhelli, G., Braicovich, L., Minola, M., Sala, M. Moretti, Mazzoli, C., Liang, Ruixing, Bonn, D. A., Hardy, W. N., Keimer, B., Sawatzky, G. A. and Hawthorn, D. G.
Abstract:
Recently, charge density wave (CDW) order in the CuO2 planes of underdoped YBa2Cu3O6+delta was detected using resonant soft x-ray scattering. An important question remains: is the chain layer responsible for this charge ordering? Here, we explore the energy and polarization dependence of the resonant scattering intensity in a detwinned sample of YBa2Cu3O6.75 with ortho-III oxygen ordering in the chain layer. We show that the ortho-III CDW order in the chains is distinct from the CDWorder in the planes. The ortho-III structure gives rise to a commensurate superlattice reflection at Q = [0.33 0 L] whose energy and polarization dependence agrees with expectations for oxygen ordering and a spatial modulation of the Cu valence in the chains. Incommensurate peaks at [0.30 0 L] and [0 0.30 L] from the CDW order in the planes are shown to be distinct in Q as well as their temperature, energy, and polarization dependence, and are thus unrelated to the structure of the chain layer. Moreover, the energy dependence of the CDW order in the planes is shown to result from a spatial modulation of energies of the Cu 2p to 3d(x2-y2) transition, similar to stripe-ordered 214 cuprates.
Reference:
Distinct Charge Orders in the Planes and Chains of Ortho-III-Ordered YBa2Cu3O6+delta Superconductors Identified by Resonant Elastic X-ray Scattering (Achkar, A. J., Sutarto, R., Mao, X., He, F., Frano, A. and Blanco-Canosa, S., Le Tacon, M., Ghiringhelli, G., Braicovich, L., Minola, M., Sala, M. Moretti, Mazzoli, C., Liang, Ruixing, Bonn, D. A., Hardy, W. N., Keimer, B., Sawatzky, G. A. and Hawthorn, D. G.), In PHYSICAL REVIEW LETTERS, AMER PHYSICAL SOC, volume 109, 2012.
Bibtex Entry:
@article{ ISI:000309905400018, Author = {Achkar, A. J. and Sutarto, R. and Mao, X. and He, F. and Frano, A. and Blanco-Canosa, S. and Le Tacon, M. and Ghiringhelli, G. and Braicovich, L. and Minola, M. and Sala, M. Moretti and Mazzoli, C. and Liang, Ruixing and Bonn, D. A. and Hardy, W. N. and Keimer, B. and Sawatzky, G. A. and Hawthorn, D. G.}, Title = {{Distinct Charge Orders in the Planes and Chains of Ortho-III-Ordered YBa2Cu3O6+delta Superconductors Identified by Resonant Elastic X-ray Scattering}}, Journal = {{PHYSICAL REVIEW LETTERS}}, Year = {{2012}}, Volume = {{109}}, Number = {{16}}, Month = {{OCT 17}}, Abstract = {{Recently, charge density wave (CDW) order in the CuO2 planes of underdoped YBa2Cu3O6+delta was detected using resonant soft x-ray scattering. An important question remains: is the chain layer responsible for this charge ordering? Here, we explore the energy and polarization dependence of the resonant scattering intensity in a detwinned sample of YBa2Cu3O6.75 with ortho-III oxygen ordering in the chain layer. We show that the ortho-III CDW order in the chains is distinct from the CDWorder in the planes. The ortho-III structure gives rise to a commensurate superlattice reflection at Q = {[}0.33 0 L] whose energy and polarization dependence agrees with expectations for oxygen ordering and a spatial modulation of the Cu valence in the chains. Incommensurate peaks at {[}0.30 0 L] and {[}0 0.30 L] from the CDW order in the planes are shown to be distinct in Q as well as their temperature, energy, and polarization dependence, and are thus unrelated to the structure of the chain layer. Moreover, the energy dependence of the CDW order in the planes is shown to result from a spatial modulation of energies of the Cu 2p to 3d(x2-y2) transition, similar to stripe-ordered 214 cuprates.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Achkar, AJ (Corresponding Author), Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. Achkar, A. J.; Mao, X.; Hawthorn, D. G., Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. Sutarto, R.; Liang, Ruixing; Bonn, D. A.; Hardy, W. N.; Sawatzky, G. A., Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. Sutarto, R.; He, F., Univ Saskatchewan, Canadian Light Source, Saskatoon, SK S7N 0X4, Canada. Frano, A.; Blanco-Canosa, S.; Le Tacon, M.; Keimer, B., Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany. Frano, A., Helmholtz Zentrum Berlin Mat & Energie, D-12489 Berlin, Germany. Ghiringhelli, G.; Braicovich, L.; Minola, M.; Mazzoli, C., Politecn Milan, CNISM, CNR SPIN, I-20133 Milan, Italy. Ghiringhelli, G.; Braicovich, L.; Minola, M.; Mazzoli, C., Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. Sala, M. Moretti, European Synchrotron Radiat Facil, F-38043 Grenoble, France.}}, DOI = {{10.1103/PhysRevLett.109.167001}}, Article-Number = {{167001}}, ISSN = {{0031-9007}}, EISSN = {{1079-7114}}, Keywords-Plus = {{T-C; FERMI-SURFACE; TEMPERATURE; LA2-XSRXCUO4; STRIPES; LAYER; SPIN}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, Author-Email = {{dhawthor@uwaterloo.ca}}, ResearcherID-Numbers = {{Mazzoli, Claudio/J-4360-2012 Hawthorn, David G/I-6491-2012 He, Feizhou/G-8493-2015 Sala, Marco Moretti/H-1034-2014 Hardy, Walter Newbold/AAN-7827-2020 Ghiringhelli, Giacomo/D-1159-2014 Moretti, Marco/AAF-9255-2019 , Le Tacon Matthieu/D-8023-2011 Blanco-Canosa, Santiago/A-2928-2015 }}, ORCID-Numbers = {{Hawthorn, David G/0000-0002-7002-0416 He, Feizhou/0000-0002-3125-1406 Sala, Marco Moretti/0000-0002-9744-9976 Ghiringhelli, Giacomo/0000-0003-0867-7748 Moretti, Marco/0000-0002-9744-9976 , Le Tacon Matthieu/0000-0002-5838-3724 Blanco-Canosa, Santiago/0000-0002-4437-5846 Minola, Matteo/0000-0003-4084-0664 Braicovich, Lucio/0000-0001-6548-9140}}, Funding-Acknowledgement = {{Canada Foundation for InnovationCanada Foundation for InnovationCGIAR; Canadian Institute for Advanced ResearchCanadian Institute for Advanced Research (CIFAR); Natural Sciences and Engineering Research Council of CanadaNatural Sciences and Engineering Research Council of CanadaCGIAR; NSERCNatural Sciences and Engineering Research Council of Canada; NRCNational Research Centre (NRC); CIHRCanadian Institutes of Health Research (CIHR); University of Saskatchewan}}, Funding-Text = {{We thank T. Senthil, A. Burkov, S. Wilkins, and K. Shen for discussions. This work was supported by the Canada Foundation for Innovation, the Canadian Institute for Advanced Research, and the Natural Sciences and Engineering Research Council of Canada. The research described in this Letter was performed at the Canadian Light Source, which is supported by NSERC, NRC, CIHR, and the University of Saskatchewan.}}, Number-of-Cited-References = {{33}}, Times-Cited = {{203}}, Usage-Count-Last-180-days = {{5}}, Usage-Count-Since-2013 = {{97}}, Journal-ISO = {{Phys. Rev. Lett.}}, Doc-Delivery-Number = {{021SJ}}, Unique-ID = {{ISI:000309905400018}}, ESI-Highly-Cited-Paper = {{Y}}, ESI-Hot-Paper = {{N}}, DA = {{2020-12-22}}, }
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