by Ghiringhelli, G., Brookes, N. B., Dallera, C., Tagliaferri, A. and Braicovich, L.
Abstract:
We present Cu L-3 edge resonant inelastic x-ray scattering (RIXS) and resonant x-ray photoemission spectroscopy (RXPS) of La2-xSrxCuO4 (x=0.0, 0.13, and 0.27). RIXS is found to be much more sensitive to the hole doping level than resonant photoemission. RIXS allows us to determine the average energy of dd excitations of both undoped and hole doped sites. The trade-off between the Raman and non-Raman spectral features depends on the doping level strongly in RIXS but weakly in RXPS. These experimental findings are consistently interpreted within a cluster model: The role of nonlocal core hole screening in the intermediate state is shown to be crucial. Nonlocal screening has an impact also on the interpretation of the L-3 x-ray absorption spectra in cuprates.
Reference:
Sensitivity to hole doping of Cu L-3 resonant spectroscopies: Inelastic x-ray scattering and photoemission of La2-xSrxCuO4 (Ghiringhelli, G., Brookes, N. B., Dallera, C., Tagliaferri, A. and Braicovich, L.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 76, 2007.
Bibtex Entry:
@article{ ISI:000249155400028, Author = {Ghiringhelli, G. and Brookes, N. B. and Dallera, C. and Tagliaferri, A. and Braicovich, L.}, Title = {{Sensitivity to hole doping of Cu L-3 resonant spectroscopies: Inelastic x-ray scattering and photoemission of La2-xSrxCuO4}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2007}}, Volume = {{76}}, Number = {{8}}, Month = {{AUG}}, Abstract = {{We present Cu L-3 edge resonant inelastic x-ray scattering (RIXS) and resonant x-ray photoemission spectroscopy (RXPS) of La2-xSrxCuO4 (x=0.0, 0.13, and 0.27). RIXS is found to be much more sensitive to the hole doping level than resonant photoemission. RIXS allows us to determine the average energy of dd excitations of both undoped and hole doped sites. The trade-off between the Raman and non-Raman spectral features depends on the doping level strongly in RIXS but weakly in RXPS. These experimental findings are consistently interpreted within a cluster model: The role of nonlocal core hole screening in the intermediate state is shown to be crucial. Nonlocal screening has an impact also on the interpretation of the L-3 x-ray absorption spectra in cuprates.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Ghiringhelli, G (Corresponding Author), INFM COHERENTIA, CNR, Piazza Leonardo Da Vinci 32, I-20133 Milan, Italy. INFM COHERENTIA, CNR, I-20133 Milan, Italy. Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. European Synchrotron Radiat Facil, F-38043 Grenoble, France. INFM SOFT, CNR, I-20133 Milan, Italy. Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. CNISM, I-20133 Milan, Italy.}}, DOI = {{10.1103/PhysRevB.76.085116}}, Article-Number = {{085116}}, ISSN = {{2469-9950}}, EISSN = {{2469-9969}}, Keywords-Plus = {{CUPRATE SUPERCONDUCTORS; ELECTRONIC-STRUCTURE; RAMAN-SCATTERING; VALENCE-BAND; L-EDGE; ABSORPTION; BI2SR2CACU2O8; THRESHOLD; LA2CUO4}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, ResearcherID-Numbers = {{Tagliaferri, Alberto/L-2903-2015 Ghiringhelli, Giacomo/D-1159-2014 Brookes, Nicholas B/C-6718-2019 }}, ORCID-Numbers = {{Tagliaferri, Alberto/0000-0001-8001-1786 Ghiringhelli, Giacomo/0000-0003-0867-7748 Brookes, Nicholas B/0000-0002-1342-9530 Braicovich, Lucio/0000-0001-6548-9140}}, Number-of-Cited-References = {{32}}, Times-Cited = {{11}}, Usage-Count-Last-180-days = {{0}}, Usage-Count-Since-2013 = {{13}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{206AD}}, Unique-ID = {{ISI:000249155400028}}, DA = {{2020-12-22}}, }
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