by Braicovich, L, van der Laan, G, Ghiringhelli, G, Tagliaferri, A and Brookes, NB
Abstract:
We present results on resonant Raman scattering (RRS) in perpendicular geometry excited with circularly polarized x rays at the Co L-3,L-2 edges in CoFe2O4 (Co ferrite) and Co metal. In this geometry the incident x-ray beam is perpendicular to the magnetization and the magnetic dichroism is only present in the RRS and not in the absorption. We compare the 3s-RRS channel terminating in an inner shell 3s hole and extra 3d electron (2p(6)3d(n)–>2p(5)3d(n+1)–>2p(6)3s(1)3d(n+1)) and the 3d-RRS channel ending in a 3d electron-hole pair (2p(6)3d(n)–>2p(5)3d(n+1)–>2p(6)3d(n)). The work is based on the measurement of the spectra vs the incident photon energy and integrated over the scattered photon energy. In both samples the dichroism of the inner-shell channel is about an order of magnitude larger than that of the valence channel. The result is explained by a theory based on the fast-collision approximation. We show that this theory provides a general way to choose the optimum scattering channel in the study of magnetic dichroism in perpendicular geometry. The impact of the results is briefly discussed.
Reference:
Magnetic circular dichroism in x-ray resonant Raman scattering in perpendicular geometry from CoFe2O4 and Co metal: A comparison of valence and inner-shell channels (Braicovich, L, van der Laan, G, Ghiringhelli, G, Tagliaferri, A and Brookes, NB), In PHYSICAL REVIEW B, AMERICAN PHYSICAL SOC, volume 66, 2002.
Bibtex Entry:
@article{ ISI:000179611700079, Author = {Braicovich, L and van der Laan, G and Ghiringhelli, G and Tagliaferri, A and Brookes, NB}, Title = {{Magnetic circular dichroism in x-ray resonant Raman scattering in perpendicular geometry from CoFe2O4 and Co metal: A comparison of valence and inner-shell channels}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2002}}, Volume = {{66}}, Number = {{17}}, Month = {{NOV 1}}, Abstract = {{We present results on resonant Raman scattering (RRS) in perpendicular geometry excited with circularly polarized x rays at the Co L-3,L-2 edges in CoFe2O4 (Co ferrite) and Co metal. In this geometry the incident x-ray beam is perpendicular to the magnetization and the magnetic dichroism is only present in the RRS and not in the absorption. We compare the 3s-RRS channel terminating in an inner shell 3s hole and extra 3d electron (2p(6)3d(n)-->2p(5)3d(n+1)-->2p(6)3s(1)3d(n+1)) and the 3d-RRS channel ending in a 3d electron-hole pair (2p(6)3d(n)-->2p(5)3d(n+1)-->2p(6)3d(n)). The work is based on the measurement of the spectra vs the incident photon energy and integrated over the scattered photon energy. In both samples the dichroism of the inner-shell channel is about an order of magnitude larger than that of the valence channel. The result is explained by a theory based on the fast-collision approximation. We show that this theory provides a general way to choose the optimum scattering channel in the study of magnetic dichroism in perpendicular geometry. The impact of the results is briefly discussed.}}, Publisher = {{AMERICAN PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Braicovich, L (Corresponding Author), Politecn Milan, INFM, Dipartimento Fis, P Leonardo da Vinci 32, I-20133 Milan, Italy. Politecn Milan, INFM, Dipartimento Fis, I-20133 Milan, Italy. SERC, Daresbury Lab, Warrington WA4 4AD, Cheshire, England. European Synchrotron Radiat Facil, F-38043 Grenoble, France.}}, DOI = {{10.1103/PhysRevB.66.174435}}, Article-Number = {{174435}}, ISSN = {{1098-0121}}, Keywords-Plus = {{EMISSION-SPECTROSCOPY; HELICAL UNDULATOR; HOLE POLARIZATION; SUM-RULES; PHOTOEMISSION; ABSORPTION; FE; IRON}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, ResearcherID-Numbers = {{Tagliaferri, Alberto/L-2903-2015 Brookes, Nicholas B/C-6718-2019 Ghiringhelli, Giacomo/D-1159-2014 van der Laan, Gerrit/Q-1662-2015 }}, ORCID-Numbers = {{Tagliaferri, Alberto/0000-0001-8001-1786 Brookes, Nicholas B/0000-0002-1342-9530 Ghiringhelli, Giacomo/0000-0003-0867-7748 van der Laan, Gerrit/0000-0001-6852-2495 Braicovich, Lucio/0000-0001-6548-9140}}, Number-of-Cited-References = {{27}}, Times-Cited = {{12}}, Usage-Count-Last-180-days = {{0}}, Usage-Count-Since-2013 = {{5}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{621VL}}, Unique-ID = {{ISI:000179611700079}}, DA = {{2020-12-22}}, }
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