by Bisogni, V., Simonelli, L., Ament, L. J. P., Forte, F. and Sala, M. Moretti, Minola, M., Huotari, S., van den Brink, J., Ghiringhelli, G., Brookes, N. B. and Braicovich, L.
Abstract:
We assess the capabilities of magnetic resonant inelastic x-ray scattering (RIXS) at the O K edge in undoped cuprates by taking La2CuO4 as a benchmark case, based on a series of RIXS measurements that we present here. By combining the experimental results with basic theory we point out the fingerprints of bimagnon excitation in the O K edge RIXS spectra. These are a dominant peak around 450 meV, the almost complete absence of dispersion both with pi and sigma polarization, and the almost constant intensity vs the transferred momentum with sigma polarization. This behavior is quite different from Cu L-3 edge RIXS giving a strongly dispersing bimagnon tending to zero at the center of the Brillouin zone. This is clearly shown by RIXS measurements at the Cu L-3 edge that we present. The Cu L-3 bimagnon spectra and those at the Cu K edge-both from the literature and from our data-however, have the same shape. These similarities and differences are understood in terms of different sampling of the bimagnon continuum. This panorama points out the unique possibilities offered by O K RIXS in the study of magnetic excitations in cuprates near the center of the BZ.
Reference:
Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O K edge. I. Assessment on La2CuO4 and comparison with the excitation at Cu L-3 and Cu K edges (Bisogni, V., Simonelli, L., Ament, L. J. P., Forte, F. and Sala, M. Moretti, Minola, M., Huotari, S., van den Brink, J., Ghiringhelli, G., Brookes, N. B. and Braicovich, L.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 85, 2012.
Bibtex Entry:
@article{ ISI:000305604600007, Author = {Bisogni, V. and Simonelli, L. and Ament, L. J. P. and Forte, F. and Sala, M. Moretti and Minola, M. and Huotari, S. and van den Brink, J. and Ghiringhelli, G. and Brookes, N. B. and Braicovich, L.}, Title = {{Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O K edge. I. Assessment on La2CuO4 and comparison with the excitation at Cu L-3 and Cu K edges}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2012}}, Volume = {{85}}, Number = {{21}}, Month = {{JUN 25}}, Abstract = {{We assess the capabilities of magnetic resonant inelastic x-ray scattering (RIXS) at the O K edge in undoped cuprates by taking La2CuO4 as a benchmark case, based on a series of RIXS measurements that we present here. By combining the experimental results with basic theory we point out the fingerprints of bimagnon excitation in the O K edge RIXS spectra. These are a dominant peak around 450 meV, the almost complete absence of dispersion both with pi and sigma polarization, and the almost constant intensity vs the transferred momentum with sigma polarization. This behavior is quite different from Cu L-3 edge RIXS giving a strongly dispersing bimagnon tending to zero at the center of the Brillouin zone. This is clearly shown by RIXS measurements at the Cu L-3 edge that we present. The Cu L-3 bimagnon spectra and those at the Cu K edge-both from the literature and from our data-however, have the same shape. These similarities and differences are understood in terms of different sampling of the bimagnon continuum. This panorama points out the unique possibilities offered by O K RIXS in the study of magnetic excitations in cuprates near the center of the BZ.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Bisogni, V (Corresponding Author), Leibniz Inst Solid State & Mat Res IFW Dresden, POB 270116, D-01171 Dresden, Germany. Bisogni, V.; Simonelli, L.; Huotari, S.; Brookes, N. B., European Synchrotron Radiat Facil, F-38043 Grenoble, France. Bisogni, V.; van den Brink, J., Leibniz Inst Solid State & Mat Res IFW Dresden, D-01171 Dresden, Germany. Ament, L. J. P.; van den Brink, J., Leiden Univ, Inst Lorenz Theoret Phys, NL-2300 RA Leiden, Netherlands. Forte, F., Univ Salerno, CNR SPIN, I-84084 Salerno, Italy. Forte, F., Univ Salerno, Dipartimento Fis ER Caianiello, I-84084 Salerno, Italy. Sala, M. Moretti; Minola, M.; Ghiringhelli, G.; Braicovich, L., Politecn Milan, CNR SPIN, Dipartimento Fis, I-20133 Milan, Italy. Huotari, S., Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland.}}, DOI = {{10.1103/PhysRevB.85.214527}}, Article-Number = {{214527}}, ISSN = {{2469-9950}}, EISSN = {{2469-9969}}, Keywords-Plus = {{FLUORESCENCE SPECTROSCOPY; RESOLUTION; SPECTROMETERS; CRYSTALS; PHONON; STATES}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, ResearcherID-Numbers = {{Sala, Marco Moretti/H-1034-2014 Simonelli, Laura/I-1963-2015 Brookes, Nicholas B/C-6718-2019 van den Brink, Jeroen/E-5670-2011 Moretti, Marco/AAF-9255-2019 van den Brink, Jeroen/Y-3931-2019 Ghiringhelli, Giacomo/D-1159-2014 }}, ORCID-Numbers = {{Sala, Marco Moretti/0000-0002-9744-9976 Brookes, Nicholas B/0000-0002-1342-9530 van den Brink, Jeroen/0000-0001-6594-9610 Moretti, Marco/0000-0002-9744-9976 Ghiringhelli, Giacomo/0000-0003-0867-7748 Braicovich, Lucio/0000-0001-6548-9140 Minola, Matteo/0000-0003-4084-0664 Huotari, Simo/0000-0003-4506-8722}}, Funding-Acknowledgement = {{Deutscher Akademischer Austausch DienstDeutscher Akademischer Austausch Dienst (DAAD); Helsinki University research funds {[}490076]; Academy of FinlandAcademy of Finland {[}1256211, 1254065]; {[}264098-MAMA]}}, Funding-Text = {{The work took enormous advantage from numerous stimulating and productive discussions with many colleagues and in particular with B. Buchner, J. Geck, J. Mesot, and G. Monaco. The Cu L<INF>3</INF> RIXS was performed at the ADRESS beam line of the SLS (PSI) using the SAXES spectrometer developed jointly by Politecnico di Milano, SLS, and EPFL. For the measurements taken at the SLS we acknowledge the assistance by T. Schmitt. The authors are grateful to F. Miletto Granozio and M. Radovic for providing the LCO thin film sample and to J. Mesot for the LCO single crystal. V.B. acknowledges the financial support from Deutscher Akademischer Austausch Dienst. F.F. acknowledges financial support from FP7/2007-2013 under Grant Agreement No. 264098-MAMA. S.H. was supported by Helsinki University research funds (Project No. 490076) and the Academy of Finland (Projects No. 1256211 and No. 1254065).}}, Number-of-Cited-References = {{45}}, Times-Cited = {{38}}, Usage-Count-Last-180-days = {{1}}, Usage-Count-Since-2013 = {{37}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{963FD}}, Unique-ID = {{ISI:000305604600007}}, DA = {{2020-12-22}}, }
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