by Minola, M., Di Castro, D., Braicovich, L., Brookes, N. B. and Innocenti, D., Sala, M. Moretti, Tebano, A. and Balestrino, G. and Ghiringhelli, G.
Abstract:
Using high-resolution resonant inelastic x-ray scattering (RIXS) excited at the Cu L-3 edge we have investigated the ligand field (dd) and magnetic excitations in (CaCuO2)(n)/(SrTiO3)(n) superlattices (n = 2,3) and compared them to those of a 14-nm-thick CaCuO2 film. The dd excitation spectrum reveals a pyramidal coordination of Cu ions at the CaCuO2/SrTiO3 interfaces. In the three samples, spin excitations are in the form of dispersing magnons, with similar spectral intensity but reduced dynamics in SLs with respect to pure CaCuO2. By fitting the dispersions within linear spin wave theory we have obtained the leading term of the in-plane superexchange parameters: J = 127 meV, 138 meV, and 157 meV for n = 2, 3 SLs, and CaCuO2, respectively. These results demonstrate that the antiferromagnetic order is preserved in these SLs down to very small cuprate layer thickness and despite the chemical and structural alterations at the interface. This finding opens the way to the production of artificial Cu-based high-temperature superconductors where the charge reservoir layer is constituted by the interface itself.
Reference:
Magnetic and ligand field properties of copper at the interfaces of (CaCuO2)(n)/(SrTiO3)(n) superlattices (Minola, M., Di Castro, D., Braicovich, L., Brookes, N. B. and Innocenti, D., Sala, M. Moretti, Tebano, A. and Balestrino, G. and Ghiringhelli, G.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 85, 2012.
Bibtex Entry:
@article{ ISI:000305533900005, Author = {Minola, M. and Di Castro, D. and Braicovich, L. and Brookes, N. B. and Innocenti, D. and Sala, M. Moretti and Tebano, A. and Balestrino, G. and Ghiringhelli, G.}, Title = {{Magnetic and ligand field properties of copper at the interfaces of (CaCuO2)(n)/(SrTiO3)(n) superlattices}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2012}}, Volume = {{85}}, Number = {{23}}, Month = {{JUN 20}}, Abstract = {{Using high-resolution resonant inelastic x-ray scattering (RIXS) excited at the Cu L-3 edge we have investigated the ligand field (dd) and magnetic excitations in (CaCuO2)(n)/(SrTiO3)(n) superlattices (n = 2,3) and compared them to those of a 14-nm-thick CaCuO2 film. The dd excitation spectrum reveals a pyramidal coordination of Cu ions at the CaCuO2/SrTiO3 interfaces. In the three samples, spin excitations are in the form of dispersing magnons, with similar spectral intensity but reduced dynamics in SLs with respect to pure CaCuO2. By fitting the dispersions within linear spin wave theory we have obtained the leading term of the in-plane superexchange parameters: J = 127 meV, 138 meV, and 157 meV for n = 2, 3 SLs, and CaCuO2, respectively. These results demonstrate that the antiferromagnetic order is preserved in these SLs down to very small cuprate layer thickness and despite the chemical and structural alterations at the interface. This finding opens the way to the production of artificial Cu-based high-temperature superconductors where the charge reservoir layer is constituted by the interface itself.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Minola, M (Corresponding Author), Politecn Milan, CNISM, I-20133 Milan, Italy. Minola, M., Politecn Milan, CNISM, I-20133 Milan, Italy. Di Castro, D.; Innocenti, D.; Tebano, A.; Balestrino, G., Univ Roma Tor Vergata, CNR SPIN, I-00133 Rome, Italy. Minola, M.; Braicovich, L.; Sala, M. Moretti; Ghiringhelli, G., Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. Di Castro, D.; Innocenti, D.; Tebano, A.; Balestrino, G., Univ Roma Tor Vergata, Dipartimento Ingn Civile & Ingn Informat, I-00133 Rome, Italy. Braicovich, L.; Sala, M. Moretti; Ghiringhelli, G., Politecn Milan, CNR SPIN, I-20133 Milan, Italy. Brookes, N. B., European Synchrotron Radiat Facil, F-38043 Grenoble, France.}}, DOI = {{10.1103/PhysRevB.85.235138}}, Article-Number = {{235138}}, ISSN = {{1098-0121}}, Keywords-Plus = {{TEMPERATURE; SUPERCONDUCTORS; CACUO2; OXIDES}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, ResearcherID-Numbers = {{Brookes, Nicholas B/C-6718-2019 Ghiringhelli, Giacomo/D-1159-2014 Sala, Marco Moretti/H-1034-2014 Moretti, Marco/AAF-9255-2019 innocenti, davide/H-7786-2012 }}, ORCID-Numbers = {{Brookes, Nicholas B/0000-0002-1342-9530 Ghiringhelli, Giacomo/0000-0003-0867-7748 Sala, Marco Moretti/0000-0002-9744-9976 Moretti, Marco/0000-0002-9744-9976 innocenti, davide/0000-0002-0465-3039 TEBANO, ANTONELLO/0000-0002-0229-671X Minola, Matteo/0000-0003-4084-0664 Braicovich, Lucio/0000-0001-6548-9140 DI CASTRO, DANIELE/0000-0002-0878-6904}}, Funding-Acknowledgement = {{Italian Ministry of Research MIURMinistry of Education, Universities and Research (MIUR) {[}PRIN-20094W2LAY]}}, Funding-Text = {{This research project has been partially supported by the Italian Ministry of Research MIUR (Grant No. PRIN-20094W2LAY).}}, Number-of-Cited-References = {{28}}, Times-Cited = {{14}}, Usage-Count-Last-180-days = {{1}}, Usage-Count-Since-2013 = {{32}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{962HN}}, Unique-ID = {{ISI:000305533900005}}, DA = {{2020-12-22}}, }
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