by Minola, M., Di Castro, D., Braicovich, L., Brookes, N. B. and Innocenti, D., Sala, M. Moretti, Tebano, A. and Balestrino, G. and Ghiringhelli, G.
Abstract:
Using high-resolution resonant inelastic x-ray scattering (RIXS) excited at the Cu L-3 edge we have investigated the ligand field (dd) and magnetic excitations in (CaCuO2)(n)/(SrTiO3)(n) superlattices (n = 2,3) and compared them to those of a 14-nm-thick CaCuO2 film. The dd excitation spectrum reveals a pyramidal coordination of Cu ions at the CaCuO2/SrTiO3 interfaces. In the three samples, spin excitations are in the form of dispersing magnons, with similar spectral intensity but reduced dynamics in SLs with respect to pure CaCuO2. By fitting the dispersions within linear spin wave theory we have obtained the leading term of the in-plane superexchange parameters: J = 127 meV, 138 meV, and 157 meV for n = 2, 3 SLs, and CaCuO2, respectively. These results demonstrate that the antiferromagnetic order is preserved in these SLs down to very small cuprate layer thickness and despite the chemical and structural alterations at the interface. This finding opens the way to the production of artificial Cu-based high-temperature superconductors where the charge reservoir layer is constituted by the interface itself.
Reference:
Magnetic and ligand field properties of copper at the interfaces of (CaCuO2)(n)/(SrTiO3)(n) superlattices (Minola, M., Di Castro, D., Braicovich, L., Brookes, N. B. and Innocenti, D., Sala, M. Moretti, Tebano, A. and Balestrino, G. and Ghiringhelli, G.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 85, 2012.
Bibtex Entry:
@article{ ISI:000305533900005,
Author = {Minola, M. and Di Castro, D. and Braicovich, L. and Brookes, N. B. and
Innocenti, D. and Sala, M. Moretti and Tebano, A. and Balestrino, G. and
Ghiringhelli, G.},
Title = {{Magnetic and ligand field properties of copper at the interfaces of
(CaCuO2)(n)/(SrTiO3)(n) superlattices}},
Journal = {{PHYSICAL REVIEW B}},
Year = {{2012}},
Volume = {{85}},
Number = {{23}},
Month = {{JUN 20}},
Abstract = {{Using high-resolution resonant inelastic x-ray scattering (RIXS) excited
at the Cu L-3 edge we have investigated the ligand field (dd) and
magnetic excitations in (CaCuO2)(n)/(SrTiO3)(n) superlattices (n = 2,3)
and compared them to those of a 14-nm-thick CaCuO2 film. The dd
excitation spectrum reveals a pyramidal coordination of Cu ions at the
CaCuO2/SrTiO3 interfaces. In the three samples, spin excitations are in
the form of dispersing magnons, with similar spectral intensity but
reduced dynamics in SLs with respect to pure CaCuO2. By fitting the
dispersions within linear spin wave theory we have obtained the leading
term of the in-plane superexchange parameters: J = 127 meV, 138 meV, and
157 meV for n = 2, 3 SLs, and CaCuO2, respectively. These results
demonstrate that the antiferromagnetic order is preserved in these SLs
down to very small cuprate layer thickness and despite the chemical and
structural alterations at the interface. This finding opens the way to
the production of artificial Cu-based high-temperature superconductors
where the charge reservoir layer is constituted by the interface itself.}},
Publisher = {{AMER PHYSICAL SOC}},
Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}},
Type = {{Article}},
Language = {{English}},
Affiliation = {{Minola, M (Corresponding Author), Politecn Milan, CNISM, I-20133 Milan, Italy.
Minola, M., Politecn Milan, CNISM, I-20133 Milan, Italy.
Di Castro, D.; Innocenti, D.; Tebano, A.; Balestrino, G., Univ Roma Tor Vergata, CNR SPIN, I-00133 Rome, Italy.
Minola, M.; Braicovich, L.; Sala, M. Moretti; Ghiringhelli, G., Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy.
Di Castro, D.; Innocenti, D.; Tebano, A.; Balestrino, G., Univ Roma Tor Vergata, Dipartimento Ingn Civile & Ingn Informat, I-00133 Rome, Italy.
Braicovich, L.; Sala, M. Moretti; Ghiringhelli, G., Politecn Milan, CNR SPIN, I-20133 Milan, Italy.
Brookes, N. B., European Synchrotron Radiat Facil, F-38043 Grenoble, France.}},
DOI = {{10.1103/PhysRevB.85.235138}},
Article-Number = {{235138}},
ISSN = {{1098-0121}},
Keywords-Plus = {{TEMPERATURE; SUPERCONDUCTORS; CACUO2; OXIDES}},
Research-Areas = {{Materials Science; Physics}},
Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics,
Condensed Matter}},
ResearcherID-Numbers = {{Brookes, Nicholas B/C-6718-2019
Ghiringhelli, Giacomo/D-1159-2014
Sala, Marco Moretti/H-1034-2014
Moretti, Marco/AAF-9255-2019
innocenti, davide/H-7786-2012
}},
ORCID-Numbers = {{Brookes, Nicholas B/0000-0002-1342-9530
Ghiringhelli, Giacomo/0000-0003-0867-7748
Sala, Marco Moretti/0000-0002-9744-9976
Moretti, Marco/0000-0002-9744-9976
innocenti, davide/0000-0002-0465-3039
TEBANO, ANTONELLO/0000-0002-0229-671X
Minola, Matteo/0000-0003-4084-0664
Braicovich, Lucio/0000-0001-6548-9140
DI CASTRO, DANIELE/0000-0002-0878-6904}},
Funding-Acknowledgement = {{Italian Ministry of Research MIURMinistry of Education, Universities and
Research (MIUR) {[}PRIN-20094W2LAY]}},
Funding-Text = {{This research project has been partially supported by the Italian
Ministry of Research MIUR (Grant No. PRIN-20094W2LAY).}},
Number-of-Cited-References = {{28}},
Times-Cited = {{14}},
Usage-Count-Last-180-days = {{1}},
Usage-Count-Since-2013 = {{32}},
Journal-ISO = {{Phys. Rev. B}},
Doc-Delivery-Number = {{962HN}},
Unique-ID = {{ISI:000305533900005}},
DA = {{2020-12-22}},
}
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