by Ristic, Z., Di Capua, R., De Luca, G. M., Chiarella, F. and Ghiringhelli, G., Cezar, J. C., Brookes, N. B., Richter, C. and Mannhart, J. and Salluzzo, M.
Abstract:
The appearance of high-mobility electrons at the LaAlO3/SrTiO3 interface has raised strong interest in the material science community and a lively debate on the origin of the phenomenon. A possible explanation is an electronic reconstruction, realizing a transfer of electrons to SrTiO3 at the interface, thereby avoiding the build-up of excessive Coulomb energy as described by the “polarization catastrophe” associated with the alternating polar layers of the LaAlO3 film. Theoretical models predict that electrons are transferred into titanium 3d(xy) interface states and, in the presence of strong correlations, generate a charge and orbital order. Here we provide experimental evidence that at room temperature the local density of states of the LaAlO3/SrTiO3 conducting interface is modulated at the nanoscale in a short-range quasiperiodic pattern, which is consistent with the appearance of an orbital (short-range) order. This result, together with the splitting of the 3d states, confirms that an electronic reconstruction drives the functional properties of the LaAlO3/SrTiO3 oxide interface. The short-range superstructure does not fully agree with the theoretical predictions. Thus, further experimental and theoretical investigations are required to understand the electronic properties of the 2D electron system realised at the LaAlO3/SrTiO3 interface. Copyright (C) EPLA, 2011
Reference:
Nanoscale modulation of the density of states at the conducting interface between LaAlO3 and SrTiO3 band insulators (Ristic, Z., Di Capua, R., De Luca, G. M., Chiarella, F. and Ghiringhelli, G., Cezar, J. C., Brookes, N. B., Richter, C. and Mannhart, J. and Salluzzo, M.), In EPL, EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY, volume 93, 2011.
Bibtex Entry:
@article{ ISI:000287024300020, Author = {Ristic, Z. and Di Capua, R. and De Luca, G. M. and Chiarella, F. and Ghiringhelli, G. and Cezar, J. C. and Brookes, N. B. and Richter, C. and Mannhart, J. and Salluzzo, M.}, Title = {{Nanoscale modulation of the density of states at the conducting interface between LaAlO3 and SrTiO3 band insulators}}, Journal = {{EPL}}, Year = {{2011}}, Volume = {{93}}, Number = {{1}}, Month = {{JAN}}, Abstract = {{The appearance of high-mobility electrons at the LaAlO3/SrTiO3 interface has raised strong interest in the material science community and a lively debate on the origin of the phenomenon. A possible explanation is an electronic reconstruction, realizing a transfer of electrons to SrTiO3 at the interface, thereby avoiding the build-up of excessive Coulomb energy as described by the ``polarization catastrophe{''} associated with the alternating polar layers of the LaAlO3 film. Theoretical models predict that electrons are transferred into titanium 3d(xy) interface states and, in the presence of strong correlations, generate a charge and orbital order. Here we provide experimental evidence that at room temperature the local density of states of the LaAlO3/SrTiO3 conducting interface is modulated at the nanoscale in a short-range quasiperiodic pattern, which is consistent with the appearance of an orbital (short-range) order. This result, together with the splitting of the 3d states, confirms that an electronic reconstruction drives the functional properties of the LaAlO3/SrTiO3 oxide interface. The short-range superstructure does not fully agree with the theoretical predictions. Thus, further experimental and theoretical investigations are required to understand the electronic properties of the 2D electron system realised at the LaAlO3/SrTiO3 interface. Copyright (C) EPLA, 2011}}, Publisher = {{EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY}}, Address = {{6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Ristic, Z (Corresponding Author), CNR SPIN, Complesso MonteSantangelo,Via Cinthia, I-80126 Naples, Italy. Ristic, Z.; Di Capua, R.; De Luca, G. M.; Chiarella, F.; Salluzzo, M., CNR SPIN, I-80126 Naples, Italy. Di Capua, R., Univ Molise, Dipartimento SpeS, I-86100 Campobasso, Italy. Ghiringhelli, G., Politecn Milan, CNR SPIN, I-20133 Milan, Italy. Ghiringhelli, G., Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. Cezar, J. C.; Brookes, N. B., European Synchrotron Radiat Facil, F-38043 Grenoble, France. Richter, C.; Mannhart, J., Univ Augsburg, Ctr Elect Correlat & Magnetism, Inst Phys, D-86135 Augsburg, Germany.}}, DOI = {{10.1209/0295-5075/93/17004}}, Article-Number = {{17004}}, ISSN = {{0295-5075}}, Keywords-Plus = {{ELECTRONIC-STRUCTURE; RECONSTRUCTION}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, Author-Email = {{salluzzo@na.infn.it}}, ResearcherID-Numbers = {{Ristic, Zoran/AAQ-6890-2020 Di Capua, Roberto/G-9622-2012 Criginski Cezar, Julio/B-2731-2008 Cezar, Julio Criginski/D-5039-2012 salluzzo, marco/C-5919-2009 Brookes, Nicholas B/C-6718-2019 Richter, Christoph/A-6172-2013 Chiarella, Fabio/G-2739-2015 Ghiringhelli, Giacomo/D-1159-2014 }}, ORCID-Numbers = {{Ristic, Zoran/0000-0002-1854-284X Di Capua, Roberto/0000-0003-3605-0993 Cezar, Julio Criginski/0000-0002-7904-6874 salluzzo, marco/0000-0001-8372-6963 Brookes, Nicholas B/0000-0002-1342-9530 Richter, Christoph/0000-0002-6591-1118 Chiarella, Fabio/0000-0003-2537-5282 Ghiringhelli, Giacomo/0000-0003-0867-7748 Mannhart, Jochen/0000-0001-6331-2640}}, Funding-Acknowledgement = {{DFGGerman Research Foundation (DFG) {[}TRR 80]; EUEuropean Union (EU)}}, Funding-Text = {{The authors are grateful to A. BARONE, M. BREITSCHAFT, S. DI MATTEO, I. MAGGIO-APRILE, J.-M. TRISCONE, and R. VAGLIO for useful discussions. Financial support by the DFG (TRR 80) and the EU (oxIDes) is gratefully acknowledged.}}, Number-of-Cited-References = {{25}}, Times-Cited = {{16}}, Usage-Count-Last-180-days = {{0}}, Usage-Count-Since-2013 = {{11}}, Journal-ISO = {{EPL}}, Doc-Delivery-Number = {{717DU}}, Unique-ID = {{ISI:000287024300020}}, DA = {{2020-12-22}}, }
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