by Hancock, J. N., Viennois, R., van der Marel, D., Ronnow, H. M., Guarise, M., Lin, P. -H., Grioni, M., Moretti Sala, M. and Ghiringhelli, G., Strocov, V. N., Schlappa, J. and Schmitt, T.
Abstract:
We present a detailed analysis of resonant inelastic x-ray scattering from Fe1.087Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition-metal L-3 edge, we observe spectra which show different characteristic features. For low-energy transfer, we experimentally observe theoretically predicted many-body effects of resonant Raman scattering from a noninteracting gas of fermions. Furthermore, we find that limitations to this many-body electron-only theory are realized at high Raman shift, where an exponential line shape reveals an energy scale not present in these considerations. This regime, identified as emission, requires considerations of lattice degrees of freedom to understand the line shape. We argue that both observations are intrinsic general features of many-body physics of metals.
Reference:
Evidence for core-hole-mediated inelastic x-ray scattering from metallic Fe1.087Te (Hancock, J. N., Viennois, R., van der Marel, D., Ronnow, H. M., Guarise, M., Lin, P. -H., Grioni, M., Moretti Sala, M. and Ghiringhelli, G., Strocov, V. N., Schlappa, J. and Schmitt, T.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 82, 2010.
Bibtex Entry:
@article{ ISI:000280229500002, Author = {Hancock, J. N. and Viennois, R. and van der Marel, D. and Ronnow, H. M. and Guarise, M. and Lin, P. -H. and Grioni, M. and Moretti Sala, M. and Ghiringhelli, G. and Strocov, V. N. and Schlappa, J. and Schmitt, T.}, Title = {{Evidence for core-hole-mediated inelastic x-ray scattering from metallic Fe1.087Te}}, Journal = {{PHYSICAL REVIEW B}}, Year = {{2010}}, Volume = {{82}}, Number = {{2}}, Month = {{JUL 23}}, Abstract = {{We present a detailed analysis of resonant inelastic x-ray scattering from Fe1.087Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition-metal L-3 edge, we observe spectra which show different characteristic features. For low-energy transfer, we experimentally observe theoretically predicted many-body effects of resonant Raman scattering from a noninteracting gas of fermions. Furthermore, we find that limitations to this many-body electron-only theory are realized at high Raman shift, where an exponential line shape reveals an energy scale not present in these considerations. This regime, identified as emission, requires considerations of lattice degrees of freedom to understand the line shape. We argue that both observations are intrinsic general features of many-body physics of metals.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Hancock, JN (Corresponding Author), Univ Geneva, Dept Phys Matiere Condensee, Quai Ernest Ansermet 24, CH-1211 Geneva 4, Switzerland. Hancock, J. N.; Viennois, R.; van der Marel, D., Univ Geneva, Dept Phys Matiere Condensee, CH-1211 Geneva 4, Switzerland. Ronnow, H. M.; Guarise, M.; Lin, P. -H.; Grioni, M., Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. Moretti Sala, M.; Ghiringhelli, G., Politecn Milan, INFM, CNR, Coherentia & Soft Dipartimento Fis, I-20133 Milan, Italy. Strocov, V. N.; Schlappa, J.; Schmitt, T., Paul Scherrer Inst, CH-5232 Villigen, Switzerland.}}, DOI = {{10.1103/PhysRevB.82.020513}}, Article-Number = {{020513}}, ISSN = {{1098-0121}}, Keywords-Plus = {{LI K-EDGE; PHONON RELAXATION; RAMAN-SCATTERING; EMISSION EDGES; ABSORPTION; SPECTRA; SINGULARITIES; SPECTROSCOPY; ELECTRON; MG}}, Research-Areas = {{Materials Science; Physics}}, Web-of-Science-Categories = {{Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter}}, ResearcherID-Numbers = {{Moretti, Marco/AAF-9255-2019 van der Marel, Dirk/G-4618-2012 Sala, Marco Moretti/H-1034-2014 Hancock, Jason/F-4694-2010 Ghiringhelli, Giacomo/D-1159-2014 Ronnow, Henrik M/A-4953-2009 Schmitt, Thorsten/A-7025-2010}}, ORCID-Numbers = {{Moretti, Marco/0000-0002-9744-9976 van der Marel, Dirk/0000-0001-5266-9847 Sala, Marco Moretti/0000-0002-9744-9976 Ghiringhelli, Giacomo/0000-0003-0867-7748 Ronnow, Henrik M/0000-0002-8832-8865 }}, Funding-Acknowledgement = {{Swiss National Science FoundationSwiss National Science Foundation (SNSF); Materials with Novel Electronic Properties (MaNEP)}}, Funding-Text = {{We would like to acknowledge valuable conversations with E. Abrahams, T. Giamarchi, G.-H. Gweon, P.M. Platzman, and B. S. Shastry and support by Swiss National Science Foundation, Materials with Novel Electronic Properties (MaNEP). ADRESS/SAXES was developed jointly by Politecnico di Milano, SLS, and EPFL.}}, Number-of-Cited-References = {{23}}, Times-Cited = {{17}}, Usage-Count-Last-180-days = {{0}}, Usage-Count-Since-2013 = {{8}}, Journal-ISO = {{Phys. Rev. B}}, Doc-Delivery-Number = {{629VY}}, Unique-ID = {{ISI:000280229500002}}, OA = {{Green Published}}, DA = {{2020-12-22}}, }
Comments are closed