by Hancock, J. N., Viennois, R., van der Marel, D., Ronnow, H. M., Guarise, M., Lin, P. -H., Grioni, M., Moretti Sala, M. and Ghiringhelli, G., Strocov, V. N., Schlappa, J. and Schmitt, T.
Abstract:
We present a detailed analysis of resonant inelastic x-ray scattering from Fe1.087Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition-metal L-3 edge, we observe spectra which show different characteristic features. For low-energy transfer, we experimentally observe theoretically predicted many-body effects of resonant Raman scattering from a noninteracting gas of fermions. Furthermore, we find that limitations to this many-body electron-only theory are realized at high Raman shift, where an exponential line shape reveals an energy scale not present in these considerations. This regime, identified as emission, requires considerations of lattice degrees of freedom to understand the line shape. We argue that both observations are intrinsic general features of many-body physics of metals.
Reference:
Evidence for core-hole-mediated inelastic x-ray scattering from metallic Fe1.087Te (Hancock, J. N., Viennois, R., van der Marel, D., Ronnow, H. M., Guarise, M., Lin, P. -H., Grioni, M., Moretti Sala, M. and Ghiringhelli, G., Strocov, V. N., Schlappa, J. and Schmitt, T.), In PHYSICAL REVIEW B, AMER PHYSICAL SOC, volume 82, 2010.
Bibtex Entry:
@article{ ISI:000280229500002,
Author = {Hancock, J. N. and Viennois, R. and van der Marel, D. and Ronnow, H. M.
   and Guarise, M. and Lin, P. -H. and Grioni, M. and Moretti Sala, M. and
   Ghiringhelli, G. and Strocov, V. N. and Schlappa, J. and Schmitt, T.},
Title = {{Evidence for core-hole-mediated inelastic x-ray scattering from metallic
   Fe1.087Te}},
Journal = {{PHYSICAL REVIEW B}},
Year = {{2010}},
Volume = {{82}},
Number = {{2}},
Month = {{JUL 23}},
Abstract = {{We present a detailed analysis of resonant inelastic x-ray scattering
   from Fe1.087Te with unprecedented energy resolution. In contrast to the
   sharp peaks typically seen in insulating systems at the transition-metal
   L-3 edge, we observe spectra which show different characteristic
   features. For low-energy transfer, we experimentally observe
   theoretically predicted many-body effects of resonant Raman scattering
   from a noninteracting gas of fermions. Furthermore, we find that
   limitations to this many-body electron-only theory are realized at high
   Raman shift, where an exponential line shape reveals an energy scale not
   present in these considerations. This regime, identified as emission,
   requires considerations of lattice degrees of freedom to understand the
   line shape. We argue that both observations are intrinsic general
   features of many-body physics of metals.}},
Publisher = {{AMER PHYSICAL SOC}},
Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}},
Type = {{Article}},
Language = {{English}},
Affiliation = {{Hancock, JN (Corresponding Author), Univ Geneva, Dept Phys Matiere Condensee, Quai Ernest Ansermet 24, CH-1211 Geneva 4, Switzerland.
   Hancock, J. N.; Viennois, R.; van der Marel, D., Univ Geneva, Dept Phys Matiere Condensee, CH-1211 Geneva 4, Switzerland.
   Ronnow, H. M.; Guarise, M.; Lin, P. -H.; Grioni, M., Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland.
   Moretti Sala, M.; Ghiringhelli, G., Politecn Milan, INFM, CNR, Coherentia & Soft Dipartimento Fis, I-20133 Milan, Italy.
   Strocov, V. N.; Schlappa, J.; Schmitt, T., Paul Scherrer Inst, CH-5232 Villigen, Switzerland.}},
DOI = {{10.1103/PhysRevB.82.020513}},
Article-Number = {{020513}},
ISSN = {{1098-0121}},
Keywords-Plus = {{LI K-EDGE; PHONON RELAXATION; RAMAN-SCATTERING; EMISSION EDGES;
   ABSORPTION; SPECTRA; SINGULARITIES; SPECTROSCOPY; ELECTRON; MG}},
Research-Areas = {{Materials Science; Physics}},
Web-of-Science-Categories  = {{Materials Science, Multidisciplinary; Physics, Applied; Physics,
   Condensed Matter}},
ResearcherID-Numbers = {{Moretti, Marco/AAF-9255-2019
   van der Marel, Dirk/G-4618-2012
   Sala, Marco Moretti/H-1034-2014
   Hancock, Jason/F-4694-2010
   Ghiringhelli, Giacomo/D-1159-2014
   Ronnow, Henrik M/A-4953-2009
   Schmitt, Thorsten/A-7025-2010}},
ORCID-Numbers = {{Moretti, Marco/0000-0002-9744-9976
   van der Marel, Dirk/0000-0001-5266-9847
   Sala, Marco Moretti/0000-0002-9744-9976
   Ghiringhelli, Giacomo/0000-0003-0867-7748
   Ronnow, Henrik M/0000-0002-8832-8865
   }},
Funding-Acknowledgement = {{Swiss National Science FoundationSwiss National Science Foundation
   (SNSF); Materials with Novel Electronic Properties (MaNEP)}},
Funding-Text = {{We would like to acknowledge valuable conversations with E. Abrahams, T.
   Giamarchi, G.-H. Gweon, P.M. Platzman, and B. S. Shastry and support by
   Swiss National Science Foundation, Materials with Novel Electronic
   Properties (MaNEP). ADRESS/SAXES was developed jointly by Politecnico di
   Milano, SLS, and EPFL.}},
Number-of-Cited-References = {{23}},
Times-Cited = {{17}},
Usage-Count-Last-180-days = {{0}},
Usage-Count-Since-2013 = {{8}},
Journal-ISO = {{Phys. Rev. B}},
Doc-Delivery-Number = {{629VY}},
Unique-ID = {{ISI:000280229500002}},
OA = {{Green Published}},
DA = {{2020-12-22}},
}

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