by Schlappa, J., Schmitt, T., Vernay, F., Strocov, V. N. and Ilakovac, V., Thielemann, B., Ronnow, H. M., Vanishri, S. and Piazzalunga, A., Wang, X., Braicovich, L., Ghiringhelli, G. and Marin, C., Mesot, J., Delley, B. and Patthey, L.
Abstract:
We investigate magnetic excitations in the spin-ladder compound Sr14Cu24O41 using high-resolution Cu L-3 edge resonant inelastic x-ray scattering (RIXS). Our findings demonstrate that RIXS couples to two-triplon collective excitations. In contrast to inelastic neutron scattering, the RIXS cross section changes only moderately over the entire Brillouin zone, revealing high sensitivity also at small momentum transfers, allowing determination of the two-triplon energy gap as 100 +/- 30 meV. Our results are backed by calculations within an effective Hubbard model for a finite-size cluster, and confirm that optical selection rules are obeyed for excitations from this spherically symmetric quantum spin-liquid ground state.
Reference:
Collective Magnetic Excitations in the Spin Ladder Sr14Cu24O41 Measured Using High-Resolution Resonant Inelastic X-Ray Scattering (Schlappa, J., Schmitt, T., Vernay, F., Strocov, V. N. and Ilakovac, V., Thielemann, B., Ronnow, H. M., Vanishri, S. and Piazzalunga, A., Wang, X., Braicovich, L., Ghiringhelli, G. and Marin, C., Mesot, J., Delley, B. and Patthey, L.), In PHYSICAL REVIEW LETTERS, AMER PHYSICAL SOC, volume 103, 2009.
Bibtex Entry:
@article{ ISI:000268307400067, Author = {Schlappa, J. and Schmitt, T. and Vernay, F. and Strocov, V. N. and Ilakovac, V. and Thielemann, B. and Ronnow, H. M. and Vanishri, S. and Piazzalunga, A. and Wang, X. and Braicovich, L. and Ghiringhelli, G. and Marin, C. and Mesot, J. and Delley, B. and Patthey, L.}, Title = {{Collective Magnetic Excitations in the Spin Ladder Sr14Cu24O41 Measured Using High-Resolution Resonant Inelastic X-Ray Scattering}}, Journal = {{PHYSICAL REVIEW LETTERS}}, Year = {{2009}}, Volume = {{103}}, Number = {{4}}, Month = {{JUL 24}}, Abstract = {{We investigate magnetic excitations in the spin-ladder compound Sr14Cu24O41 using high-resolution Cu L-3 edge resonant inelastic x-ray scattering (RIXS). Our findings demonstrate that RIXS couples to two-triplon collective excitations. In contrast to inelastic neutron scattering, the RIXS cross section changes only moderately over the entire Brillouin zone, revealing high sensitivity also at small momentum transfers, allowing determination of the two-triplon energy gap as 100 +/- 30 meV. Our results are backed by calculations within an effective Hubbard model for a finite-size cluster, and confirm that optical selection rules are obeyed for excitations from this spherically symmetric quantum spin-liquid ground state.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Schlappa, J (Corresponding Author), Paul Scherrer Inst, CH-5232 Villigen, Switzerland. Schlappa, J.; Schmitt, T.; Vernay, F.; Strocov, V. N.; Thielemann, B.; Mesot, J.; Delley, B.; Patthey, L., Paul Scherrer Inst, CH-5232 Villigen, Switzerland. Ilakovac, V., Univ Paris 06, CNRS, LCP MR, UMR 7614, Paris, France. Ilakovac, V., Univ Cergy Pontoise, Dept Phys, F-95000 Cergy Pontoise, France. Thielemann, B.; Mesot, J., ETH, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. Ronnow, H. M.; Wang, X.; Mesot, J., Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. Vanishri, S.; Marin, C., CEA, DRFMC, SPSMS, INAC, F-38054 Grenoble 9, France. Piazzalunga, A.; Braicovich, L.; Ghiringhelli, G., Politecn Milan, CNR, INFM Coherentia Soft, Dip Fis, I-20133 Milan, Italy.}}, DOI = {{10.1103/PhysRevLett.103.047401}}, Article-Number = {{047401}}, ISSN = {{0031-9007}}, Keywords-Plus = {{ELECTRONIC-STRUCTURE; SUPERCONDUCTIVITY; CHARGE; DYNAMICS}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, Author-Email = {{thorsten.schmitt@psi.ch}}, ResearcherID-Numbers = {{Ghiringhelli, Giacomo/D-1159-2014 Schmitt, Thorsten/A-7025-2010 Patthey, Luc/G-6130-2018 Ronnow, Henrik M/A-4953-2009 Delley, Bernard/E-1336-2014 }}, ORCID-Numbers = {{Ghiringhelli, Giacomo/0000-0003-0867-7748 Patthey, Luc/0000-0001-6101-8069 Ronnow, Henrik M/0000-0002-8832-8865 Delley, Bernard/0000-0002-7020-2869 Vernay, Francois/0000-0003-3713-7724 Braicovich, Lucio/0000-0001-6548-9140}}, Funding-Acknowledgement = {{Swiss NSFSwiss National Science Foundation (SNSF); Indo-FrenchFrench National Research Agency (ANR) {[}3408-4]}}, Funding-Text = {{This work was performed at the ADRESS beam line of the SLS (Paul Scherrer Institut) using the SAXES spectrometer developed jointly by Politecnico di Milano, SLS and EPFL. We gratefully acknowledge M. Kropf, J. Krempasky, and K. J. Zhou for their technical support, M. Grioni and C. Dallera for their contribution to commissioning of the SAXES spectrometer and C. Quitman for his critical reading of the manuscript. Work at the EPFL is supported by the Swiss NSF and work at CEA-Grenoble by the Indo-French project 3408-4.}}, Number-of-Cited-References = {{36}}, Times-Cited = {{85}}, Usage-Count-Last-180-days = {{1}}, Usage-Count-Since-2013 = {{35}}, Journal-ISO = {{Phys. Rev. Lett.}}, Doc-Delivery-Number = {{474TQ}}, Unique-ID = {{ISI:000268307400067}}, OA = {{Green Accepted}}, DA = {{2020-12-22}}, }
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