by Salluzzo, M., Cezar, J. C., Brookes, N. B., Bisogni, V., De Luca, G. M., Richter, C., Thiel, S., Mannhart, J., Huijben, M., Brinkman, A., Rijnders, G. and Ghiringhelli, G.
Abstract:
In 2004, Ohtomo and Hwang discovered that an electron gas is created at the interface between insulating LaAlO3 and SrTiO3 compounds. Here we show that the generation of a conducting electron gas is related to an orbital reconstruction occurring at the LaAlO3/SrTiO3 interface. Our results are based on extensive investigations of the electronic properties and of the orbital structure of the interface using x-ray absorption spectroscopy. In particular, we find that the degeneracy of the Ti 3d states is fully removed and that the Ti 3d(xy) levels become the first available states for conducting electrons.
Reference:
Orbital Reconstruction and the Two-Dimensional Electron Gas at the LaAlO3/SrTiO3 Interface (Salluzzo, M., Cezar, J. C., Brookes, N. B., Bisogni, V., De Luca, G. M., Richter, C., Thiel, S., Mannhart, J., Huijben, M., Brinkman, A., Rijnders, G. and Ghiringhelli, G.), In PHYSICAL REVIEW LETTERS, AMER PHYSICAL SOC, volume 102, 2009.
Bibtex Entry:
@article{ ISI:000265479300055, Author = {Salluzzo, M. and Cezar, J. C. and Brookes, N. B. and Bisogni, V. and De Luca, G. M. and Richter, C. and Thiel, S. and Mannhart, J. and Huijben, M. and Brinkman, A. and Rijnders, G. and Ghiringhelli, G.}, Title = {{Orbital Reconstruction and the Two-Dimensional Electron Gas at the LaAlO3/SrTiO3 Interface}}, Journal = {{PHYSICAL REVIEW LETTERS}}, Year = {{2009}}, Volume = {{102}}, Number = {{16}}, Month = {{APR 24}}, Abstract = {{In 2004, Ohtomo and Hwang discovered that an electron gas is created at the interface between insulating LaAlO3 and SrTiO3 compounds. Here we show that the generation of a conducting electron gas is related to an orbital reconstruction occurring at the LaAlO3/SrTiO3 interface. Our results are based on extensive investigations of the electronic properties and of the orbital structure of the interface using x-ray absorption spectroscopy. In particular, we find that the degeneracy of the Ti 3d states is fully removed and that the Ti 3d(xy) levels become the first available states for conducting electrons.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Salluzzo, M (Corresponding Author), CNR, INFM, COHERNTIA, Complesso MonteSantangelo Via Cinthia, I-80126 Naples, Italy. Salluzzo, M.; De Luca, G. M., CNR, INFM, COHERNTIA, I-80126 Naples, Italy. Cezar, J. C.; Brookes, N. B.; Bisogni, V., European Synchrotron Radiat Facil, F-38043 Grenoble, France. Richter, C.; Thiel, S.; Mannhart, J., Univ Augsburg, Ctr Elect Correlat & Magnetism, D-86135 Augsburg, Germany. Huijben, M.; Brinkman, A.; Rijnders, G., Univ Twente, Fac Sci & Technol, NL-7500 AE Enschede, Netherlands. Huijben, M.; Brinkman, A.; Rijnders, G., Univ Twente, MESA Inst Nanotechnol, NL-7500 AE Enschede, Netherlands. Ghiringhelli, G., CNR, INFM, COHERNTIA, I-20133 Milan, Italy. Ghiringhelli, G., Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy.}}, DOI = {{10.1103/PhysRevLett.102.166804}}, Article-Number = {{166804}}, ISSN = {{0031-9007}}, Keywords-Plus = {{X-RAY-ABSORPTION; OXIDE INTERFACES; HETEROSTRUCTURES; INSULATORS}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, Author-Email = {{salluzzo@na.infn.it}}, ResearcherID-Numbers = {{Huijben, Mark/J-7630-2017 Cezar, Julio Criginski/D-5039-2012 Brookes, Nicholas B/C-6718-2019 salluzzo, marco/C-5919-2009 Richter, Christoph/A-6172-2013 Criginski Cezar, Julio/B-2731-2008 Ghiringhelli, Giacomo/D-1159-2014 }}, ORCID-Numbers = {{Huijben, Mark/0000-0001-8175-6958 Cezar, Julio Criginski/0000-0002-7904-6874 Brookes, Nicholas B/0000-0002-1342-9530 salluzzo, marco/0000-0001-8372-6963 Richter, Christoph/0000-0002-6591-1118 Ghiringhelli, Giacomo/0000-0003-0867-7748 Mannhart, Jochen/0000-0001-6331-2640}}, Funding-Acknowledgement = {{EUEuropean Union (EU) {[}033191]; German Science FoundationGerman Research Foundation (DFG) {[}SFB 484]}}, Funding-Text = {{The authors acknowledge support from the EU under the project Nanoxide, Contract No. 033191. J. M., S. T., and C. R. gratefully acknowledge support by the German Science Foundation (SFB 484). The authors are grateful to J.-M. Triscone, R. Claessen, H. Hilgenkamp, D. H. A. Blank, R. Vaglio, and A. Barone for useful discussions.}}, Number-of-Cited-References = {{30}}, Times-Cited = {{237}}, Usage-Count-Last-180-days = {{4}}, Usage-Count-Since-2013 = {{127}}, Journal-ISO = {{Phys. Rev. Lett.}}, Doc-Delivery-Number = {{437IC}}, Unique-ID = {{ISI:000265479300055}}, DA = {{2020-12-22}}, }
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