by Yamasaki, A, Imada, S, Sekiyama, A, Tsunekawa, M, Dallera, C, Braicovich, L, Lee, TL, Sugawara, H, Sato, H, Settai, R, Onuki, Y and Suga, S
Abstract:
Bulk-sensitive photoemission spectroscopy using hard x-ray up to h nu = 5450 eV has been performed for heavy-fermion Pr compounds. A significant spectral intensity of the |3(9)4f(3)> final state was observed in Pr 3d core-level spectra of PrFe4P12 at both h nu = 2450 and 5450 eV. The spectra obtained by the configuration-interaction cluster model calculation reproduce the experimental spectra for well-hybridized PrFe4P1, and localized Pr metal. Results of the calculations suggest that the Kondo behavior observed in PrFe4P12 arise from the mixing of the |4f(2)> and |4f(3)> configurations due to the c-f hybridization. Whereas a contribution possibly from a disordered surface to the spectrum can be the fractured PrFe4P12, they cannot be disregarded for the scraped PrSn3 and Pr metal even negligible for the in the high-energy x-ray region.
Reference:
Bulk-sensitive photoemission spectroscopy for heavy-fermion Pr compounds using hard x-ray (Yamasaki, A, Imada, S, Sekiyama, A, Tsunekawa, M, Dallera, C, Braicovich, L, Lee, TL, Sugawara, H, Sato, H, Settai, R, Onuki, Y and Suga, S), In JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, PHYSICAL SOC JAPAN, volume 74, 2005.
Bibtex Entry:
@article{ ISI:000230659300034, Author = {Yamasaki, A and Imada, S and Sekiyama, A and Tsunekawa, M and Dallera, C and Braicovich, L and Lee, TL and Sugawara, H and Sato, H and Settai, R and Onuki, Y and Suga, S}, Title = {{Bulk-sensitive photoemission spectroscopy for heavy-fermion Pr compounds using hard x-ray}}, Journal = {{JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN}}, Year = {{2005}}, Volume = {{74}}, Number = {{7}}, Pages = {{2045-2051}}, Month = {{JUL}}, Abstract = {{Bulk-sensitive photoemission spectroscopy using hard x-ray up to h nu = 5450 eV has been performed for heavy-fermion Pr compounds. A significant spectral intensity of the |3(9)4f(3)> final state was observed in Pr 3d core-level spectra of PrFe4P12 at both h nu = 2450 and 5450 eV. The spectra obtained by the configuration-interaction cluster model calculation reproduce the experimental spectra for well-hybridized PrFe4P1, and localized Pr metal. Results of the calculations suggest that the Kondo behavior observed in PrFe4P12 arise from the mixing of the |4f(2)> and |4f(3)> configurations due to the c-f hybridization. Whereas a contribution possibly from a disordered surface to the spectrum can be the fractured PrFe4P12, they cannot be disregarded for the scraped PrSn3 and Pr metal even negligible for the in the high-energy x-ray region.}}, Publisher = {{PHYSICAL SOC JAPAN}}, Address = {{YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Yamasaki, A (Corresponding Author), Osaka Univ, Grad Sch Engn Sci, Toyonaka, Osaka 5608531, Japan. Osaka Univ, Grad Sch Engn Sci, Toyonaka, Osaka 5608531, Japan. Politecn Milan, Dipartimento Fis, INFM, I-20133 Milan, Italy. European Synchrotron Radiat Facil, F-38043 Grenoble, France. Tokyo Metropolitan Univ, Grad Sch Sci, Tokyo 1920397, Japan. Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan.}}, DOI = {{10.1143/JPSJ.74.2045}}, ISSN = {{0031-9015}}, Keywords = {{hard x-ray; photoemission spectroscopy; bulk sensitive; Pr compounds; heavy fermions}}, Keywords-Plus = {{RESOLUTION RESONANCE PHOTOEMISSION; 4F ELECTRONIC STATES; RARE-EARTH; CE COMPOUNDS; SPECTRA; PRFE4P12; INTERMETALLICS; METAL; ND}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, Author-Email = {{vaniasaki@decima.mp.es.osaka-u.ac.jp}}, ResearcherID-Numbers = {{Imada, Shin/F-1113-2014 Sekiyama, Akira/G-1851-2016 }}, ORCID-Numbers = {{Braicovich, Lucio/0000-0001-6548-9140}}, Number-of-Cited-References = {{39}}, Times-Cited = {{9}}, Usage-Count-Last-180-days = {{0}}, Usage-Count-Since-2013 = {{5}}, Journal-ISO = {{J. Phys. Soc. Jpn.}}, Doc-Delivery-Number = {{947PU}}, Unique-ID = {{ISI:000230659300034}}, DA = {{2020-12-22}}, }
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