by Haverkort, MW, Hu, Z, Tanaka, A, Ghiringhelli, G, Roth, H, Cwik, M, Lorenz, T, Schussler-Langeheine, C, Streltsov, SV, Mylnikova, AS, Anisimov, VI, de Nadai, C, Brookes, NB and Hsieh, HH, Lin, HJ, Chen, CT, Mizokawa, T, Taguchi, Y and Tokura, Y, Khomskii, DI and Tjeng, LH
Abstract:
Utilizing a sum rule in a spin-resolved photoelectron spectroscopic experiment with circularly polarized light, we show that the orbital moment in LaTiO3 is strongly reduced from its ionic value, both below and above the Neel temperature. Using Ti L-2,L-3 x-ray absorption spectroscopy as a local probe, we found that the crystal-field splitting in the t(2g) subshell is about 0.12-0.30 eV. This large splitting does not facilitate the formation of an orbital liquid.
Reference:
Determination of the orbital moment and crystal-field splitting in LaTiO3 (Haverkort, MW, Hu, Z, Tanaka, A, Ghiringhelli, G, Roth, H, Cwik, M, Lorenz, T, Schussler-Langeheine, C, Streltsov, SV, Mylnikova, AS, Anisimov, VI, de Nadai, C, Brookes, NB and Hsieh, HH, Lin, HJ, Chen, CT, Mizokawa, T, Taguchi, Y and Tokura, Y, Khomskii, DI and Tjeng, LH), In PHYSICAL REVIEW LETTERS, AMER PHYSICAL SOC, volume 94, 2005.
Bibtex Entry:
@article{ ISI:000226941500053,
Author = {Haverkort, MW and Hu, Z and Tanaka, A and Ghiringhelli, G and Roth, H
and Cwik, M and Lorenz, T and Schussler-Langeheine, C and Streltsov, SV
and Mylnikova, AS and Anisimov, VI and de Nadai, C and Brookes, NB and
Hsieh, HH and Lin, HJ and Chen, CT and Mizokawa, T and Taguchi, Y and
Tokura, Y and Khomskii, DI and Tjeng, LH},
Title = {{Determination of the orbital moment and crystal-field splitting in
LaTiO3}},
Journal = {{PHYSICAL REVIEW LETTERS}},
Year = {{2005}},
Volume = {{94}},
Number = {{5}},
Month = {{FEB 11}},
Abstract = {{Utilizing a sum rule in a spin-resolved photoelectron spectroscopic
experiment with circularly polarized light, we show that the orbital
moment in LaTiO3 is strongly reduced from its ionic value, both below
and above the Neel temperature. Using Ti L-2,L-3 x-ray absorption
spectroscopy as a local probe, we found that the crystal-field splitting
in the t(2g) subshell is about 0.12-0.30 eV. This large splitting does
not facilitate the formation of an orbital liquid.}},
Publisher = {{AMER PHYSICAL SOC}},
Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}},
Type = {{Article}},
Language = {{English}},
Affiliation = {{Haverkort, MW (Corresponding Author), Univ Cologne, Inst Phys 2, Zulpicher Str 77, D-50937 Cologne, Germany.
Univ Cologne, Inst Phys 2, D-50937 Cologne, Germany.
Hiroshima Univ, Dept Quantum Matter, ADSM, Higashihiroshima 7398530, Japan.
Politecn Milan, INFM, Dipartimento Fis, I-20133 Milan, Italy.
Inst Met Phys, Ekaterinburg 620219, Russia.
European Synchrotron Radiat Facil, F-38043 Grenoble, France.
Natl Def Univ, Chung Cheng Inst Technol, Taoyuan 335, Taiwan.
Natl Synchrotron Radiat Res Ctr, Hsinchu 30077, Taiwan.
Univ Tokyo, Dept Complex Sci & Engn, Tokyo 1130033, Japan.
Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan.
AIST, Japan Sci & Technol Corp, ERATO, Spin Superstruct Project, Tsukuba, Ibaraki 3058562, Japan.}},
DOI = {{10.1103/PhysRevLett.94.056401}},
Article-Number = {{056401}},
ISSN = {{0031-9007}},
EISSN = {{1079-7114}},
Keywords-Plus = {{X-RAY-ABSORPTION; ELECTRONIC-STRUCTURE; PHOTOEMISSION; OXIDES;
DICHROISM; SYSTEMS; STATES; 3D}},
Research-Areas = {{Physics}},
Web-of-Science-Categories = {{Physics, Multidisciplinary}},
ResearcherID-Numbers = {{Brookes, Nicholas B/C-6718-2019
Lorenz, Thomas/AAC-3331-2020
Haverkort, Maurits W./D-2319-2009
Hu, Zhiwei/B-8635-2008
Taguchi, Yasujiro/A-3048-2010
Tokura, Yoshinori/C-7352-2009
Lorenz, Thomas/J-2955-2017
Mizokawa, Takashi/E-3302-2015
Tjeng, Liu Hao/B-8607-2019
Anisimov, Vladimir/K-1235-2013
Streltsov, Sergey/A-6674-2012
Ghiringhelli, Giacomo/D-1159-2014
Streltsov, Sergey/A-8293-2016
SchuSSler-Langeheine, Christian/C-3186-2008
Tanaka, Arata/S-4466-2018}},
ORCID-Numbers = {{Brookes, Nicholas B/0000-0002-1342-9530
Lorenz, Thomas/0000-0003-4832-5157
Haverkort, Maurits W./0000-0002-7216-3146
Tokura, Yoshinori/0000-0002-2732-4983
Lorenz, Thomas/0000-0003-4832-5157
Mizokawa, Takashi/0000-0002-7682-2348
Tjeng, Liu Hao/0000-0002-0595-9312
Anisimov, Vladimir/0000-0002-1087-1956
Streltsov, Sergey/0000-0002-2823-1754
Ghiringhelli, Giacomo/0000-0003-0867-7748
SchuSSler-Langeheine, Christian/0000-0002-4553-9726
Tanaka, Arata/0000-0001-8301-8502}},
Funding-Acknowledgement = {{Grants-in-Aid for Scientific ResearchMinistry of Education, Culture,
Sports, Science and Technology, Japan (MEXT)Japan Society for the
Promotion of ScienceGrants-in-Aid for Scientific Research (KAKENHI)
{[}15340106, 16540318] Funding Source: KAKEN}},
Number-of-Cited-References = {{21}},
Times-Cited = {{52}},
Usage-Count-Last-180-days = {{0}},
Usage-Count-Since-2013 = {{45}},
Journal-ISO = {{Phys. Rev. Lett.}},
Doc-Delivery-Number = {{896NT}},
Unique-ID = {{ISI:000226941500053}},
DA = {{2020-12-22}},
}
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