by Brookes, NB, Ghiringhelli, G, Tjernberg, O, Tjeng, LH and Mizokawa, T, Li, TW and Menovsky, AA
Abstract:
From a spin-resolved photoemission study on the Bi2Sr2CaCu2O8+delta superconductor, we show experimentally that the first ionization state is of nearly pure singlet character. This is true both above and below the superconducting transition and in the presence of doping and band formation. This provides direct support for the existence and stability of Zhang-Rice singlets in high-temperature superconductors, justifying the ansatz of single-band models. Moreover, we establish this technique as an important probe for a wide range of cuprates and strongly correlated materials.
Reference:
Detection of Zhang-Rice singlets using spin-polarized photoemission (Brookes, NB, Ghiringhelli, G, Tjernberg, O, Tjeng, LH and Mizokawa, T, Li, TW and Menovsky, AA), In PHYSICAL REVIEW LETTERS, AMER PHYSICAL SOC, volume 87, 2001.
Bibtex Entry:
@article{ ISI:000172545400039, Author = {Brookes, NB and Ghiringhelli, G and Tjernberg, O and Tjeng, LH and Mizokawa, T and Li, TW and Menovsky, AA}, Title = {{Detection of Zhang-Rice singlets using spin-polarized photoemission}}, Journal = {{PHYSICAL REVIEW LETTERS}}, Year = {{2001}}, Volume = {{87}}, Number = {{23}}, Month = {{DEC 3}}, Abstract = {{From a spin-resolved photoemission study on the Bi2Sr2CaCu2O8+delta superconductor, we show experimentally that the first ionization state is of nearly pure singlet character. This is true both above and below the superconducting transition and in the presence of doping and band formation. This provides direct support for the existence and stability of Zhang-Rice singlets in high-temperature superconductors, justifying the ansatz of single-band models. Moreover, we establish this technique as an important probe for a wide range of cuprates and strongly correlated materials.}}, Publisher = {{AMER PHYSICAL SOC}}, Address = {{ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA}}, Type = {{Article}}, Language = {{English}}, Affiliation = {{Brookes, NB (Corresponding Author), European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. European Synchrotron Radiat Facil, F-38043 Grenoble, France. Univ Groningen, Ctr Mat Sci, Solid State Phys Lab, NL-9747 AG Groningen, Netherlands. Univ Amsterdam, Van der Waals Zeeman Lab, NL-1018 XE Amsterdam, Netherlands.}}, DOI = {{10.1103/PhysRevLett.87.237003}}, Article-Number = {{237003}}, ISSN = {{0031-9007}}, EISSN = {{1079-7114}}, Keywords-Plus = {{HIGH-TC SUPERCONDUCTIVITY; ELECTRONIC-STRUCTURE; RESONANT-PHOTOEMISSION; J MODEL; LA2-XSRXCUO4; STABILITY; VALIDITY; LA2CUO4; STATES; PLANE}}, Research-Areas = {{Physics}}, Web-of-Science-Categories = {{Physics, Multidisciplinary}}, ResearcherID-Numbers = {{Tjeng, Liu Hao/B-8607-2019 Ghiringhelli, Giacomo/D-1159-2014 Brookes, Nicholas B/C-6718-2019 Mizokawa, Takashi/E-3302-2015 }}, ORCID-Numbers = {{Tjeng, Liu Hao/0000-0002-0595-9312 Ghiringhelli, Giacomo/0000-0003-0867-7748 Brookes, Nicholas B/0000-0002-1342-9530 Mizokawa, Takashi/0000-0002-7682-2348 Tjernberg, Oscar/0000-0001-8669-6886}}, Number-of-Cited-References = {{37}}, Times-Cited = {{28}}, Usage-Count-Last-180-days = {{2}}, Usage-Count-Since-2013 = {{6}}, Journal-ISO = {{Phys. Rev. Lett.}}, Doc-Delivery-Number = {{498ZZ}}, Unique-ID = {{ISI:000172545400039}}, DA = {{2020-12-22}}, }
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